English

Gapless spin-liquid state in the structurally disorder-free triangular antiferromagnet NaYbO$_2$

Strongly Correlated Electrons 2021-01-13 v1 Materials Science

Abstract

We present the structural characterization and low-temperature magnetism of the triangular-lattice delafossite NaYbO2_2. Synchrotron x-ray diffraction and neutron scattering exclude both structural disorder and crystal-electric-field randomness, whereas heat-capacity measurements and muon spectroscopy reveal the absence of magnetic order and persistent spin dynamics down to at least 70\,mK. Continuous magnetic excitations with the low-energy spectral weight accumulating at the KK-point of the Brillouin zone indicate the formation of a novel spin-liquid phase in a triangular antiferromagnet. This phase is gapless and shows a non-trivial evolution of the low-temperature specific heat. Our work demonstrates that NaYbO2_2 practically gives the most direct experimental access to the spin-liquid physics of triangular antiferromagnets.

Keywords

Cite

@article{arxiv.1901.07810,
  title  = {Gapless spin-liquid state in the structurally disorder-free triangular antiferromagnet NaYbO$_2$},
  author = {Lei Ding and Pascal Manuel and Sebastian Bachus and Franziska Grußler and Philipp Gegenwart and John Singleton and Roger D. Johnson and Helen C. Walker and Devashibhai T. Adroja and Adrian D. Hillier and Alexander A. Tsirlin},
  journal= {arXiv preprint arXiv:1901.07810},
  year   = {2021}
}

Comments

6 pages, 4figures

R2 v1 2026-06-23T07:19:34.417Z