We investigate the physical properties of a single crystal of uranium telluride U7Te12. We have confirmed that U7Te12 crystallizes in the hexagonal structure with three nonequivalent crystallographic uranium sites. The paramagnetic moments are estimated to be approximately 1 μB per the uranium site, assuming a uniform moment on all the sites. A ferromagnetic phase transition occurs at TC=48 K, where the in-plane magnetization increases sharply, whereas the out-of-plane component does not increase significantly. With decreasing temperature further below TC under field-cooling conditions, the out-of-plane component increases rapidly around T⋆=26 K. In contrast, the in-plane component hardly changes at T⋆. Specific heat measurement indicates no λ-type anomaly around T⋆, so this is a cross-over suggesting a reorientation of the ordering moments or successive magnetic ordering on the part of the multiple uranium sites.
@article{arxiv.2211.16760,
title = {Ferromagnetic Crossover within the Ferromagnetic Order of U$_{7}$Te$_{12}$},
author = {Petr Opletal and Hironori Sakai and Yoshinori Haga and Yoshifumi Tokiwa and Etsuji Yamamoto and Shinsaku Kambe and Yo Tokunaga},
journal= {arXiv preprint arXiv:2211.16760},
year = {2023}
}