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Ferromagnetic Crossover within the Ferromagnetic Order of U$_{7}$Te$_{12}$

Strongly Correlated Electrons 2023-02-17 v1 Materials Science

Abstract

We investigate the physical properties of a single crystal of uranium telluride U7_{7}Te12_{12}. We have confirmed that U7_{7}Te12_{12} crystallizes in the hexagonal structure with three nonequivalent crystallographic uranium sites. The paramagnetic moments are estimated to be approximately 1 μB\mu_{\rm B} per the uranium site, assuming a uniform moment on all the sites. A ferromagnetic phase transition occurs at TC=48T_{\rm C}=48 K, where the in-plane magnetization increases sharply, whereas the out-of-plane component does not increase significantly. With decreasing temperature further below TCT_{\rm C} under field-cooling conditions, the out-of-plane component increases rapidly around T=26T^{\star}=26 K. In contrast, the in-plane component hardly changes at TT^{\star}. Specific heat measurement indicates no λ\lambda-type anomaly around TT^{\star}, so this is a cross-over suggesting a reorientation of the ordering moments or successive magnetic ordering on the part of the multiple uranium sites.

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Cite

@article{arxiv.2211.16760,
  title  = {Ferromagnetic Crossover within the Ferromagnetic Order of U$_{7}$Te$_{12}$},
  author = {Petr Opletal and Hironori Sakai and Yoshinori Haga and Yoshifumi Tokiwa and Etsuji Yamamoto and Shinsaku Kambe and Yo Tokunaga},
  journal= {arXiv preprint arXiv:2211.16760},
  year   = {2023}
}