Electric field dependence of complex-dominated ultracold molecular collisions
Abstract
Recent experiments on ultracold non-reactive dipolar molecules have observed high two-body losses, even though these molecules can undergo neither inelastic, nor reactive (as they are in their absolute ground state), nor light-assisted collisions (if they are measured in the dark). In the presence of an electric field these losses seem to be near universal (the probability of loss at short-range is near unity) while in the absence of it the losses seem non-universal. To explain these observations we propose a simple model based on the mixing effect of an electric field on the states of the two diatomic molecules at long-range and on the density-of-states of the tetramer complex formed at short-range, believed to be responsible for the losses. We apply our model to collisions of ground-state molecules of endothermic systems, of current experimental interest.
Keywords
Cite
@article{arxiv.2109.02602,
title = {Electric field dependence of complex-dominated ultracold molecular collisions},
author = {Goulven Quéméner and James F. E. Croft and John L. Bohn},
journal= {arXiv preprint arXiv:2109.02602},
year = {2024}
}