English

Dynamical Heterogeneities and Cooperative Motion in Smectic Liquid Crystals

Soft Condensed Matter 2009-12-15 v1

Abstract

Using simulations of hard rods in smectic-A states, we find non-gaussian diffusion and heterogeneous dynamics due to the equilibrium periodic smectic density profiles, which give rise to permanent barriers for layer-to-layer diffusion. This relaxation behavior is surprisingly similar to that of non-equilibrium supercooled liquids, although there the particles are trapped in transient (instead of permanent) cages. Interestingly, we also find stringlike clusters of up to 10 inter-layer rods exhibiting dynamic cooperativity in this equilibrium state.

Keywords

Cite

@article{arxiv.0906.3093,
  title  = {Dynamical Heterogeneities and Cooperative Motion in Smectic Liquid Crystals},
  author = {A. Patti and D. El Masri and R. van Roij and M. Dijkstra},
  journal= {arXiv preprint arXiv:0906.3093},
  year   = {2009}
}

Comments

10 pages, 4 figures

R2 v1 2026-06-21T13:14:08.616Z