Disentangle pathways in strong field molecular photoionization byangular distribution of dissociation fragments
Abstract
In strong field ionization, the pump pulse not only photoionizes the molecule, but also drives efficient population exchanges between its ionic ground and excited states.In this study, we investigated the population dynamics accompanying strong field molecular photoionization, using angular distribution of dissociative fragments after ionization.Our results reveal that the first and higher order processes of the post-ionization population redistribution mechanism (PPRM) in the ion core can be disentangled and classified by {its} angle-resolved kinetic energy release (KER) spectra.We demonstrate that the imprints of PPRM in the KER spectra can be used to determine the branching ratio of the population exchange pathways of different orders, by exploiting the pump intensity dependent variation of the spectra.
Keywords
Cite
@article{arxiv.2107.06763,
title = {Disentangle pathways in strong field molecular photoionization byangular distribution of dissociation fragments},
author = {Xiangxu Mu and Ming Zhang and Hanwei Yang and Haitan Xu and Song Bin Zhang and Lushuai Cao and Min Li and Zijian Lü and Chengyin Wu and Zheng Li},
journal= {arXiv preprint arXiv:2107.06763},
year = {2021}
}