English

Dependence of the glass transition and jamming densities on spatial dimension

Soft Condensed Matter 2022-04-07 v1 Disordered Systems and Neural Networks Statistical Mechanics

Abstract

We investigate the dynamics of soft sphere liquids through computer simulations for spatial dimensions from d=3d =3 to 88, over a wide range of temperatures and densities. Employing a scaling of density-temperature dependent relaxation times, we precisely identify the density ϕ0\phi_0 which marks the ideal glass transition in the hard sphere limit, and a crossover from sub- to super-Arrhenius temperature dependence. The difference between ϕ0\phi_0 and the athermal jamming density ϕJ\phi_J, small in 3 and 4 dimensions, increases with dimension, with ϕ0>ϕJ\phi_0 > \phi_J for d>4d > 4. We compare our results with recent theoretical calculations.

Keywords

Cite

@article{arxiv.2204.02936,
  title  = {Dependence of the glass transition and jamming densities on spatial dimension},
  author = {Monoj Adhikari and Smarajit Karmakar and Srikanth Sastry},
  journal= {arXiv preprint arXiv:2204.02936},
  year   = {2022}
}

Comments

Supplemental Material included as ancillary file