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Cuprates phase diagram deduced from magnetic susceptibility: what is the `true' pseudogap line?

Superconductivity 2022-04-06 v1 Strongly Correlated Electrons

Abstract

Two contradictory phase diagrams have dominated the literature of high-TcT_c cuprate superconductors. Does the pseudogap line cross the superconducting TcT_c-dome or not? To answer, we have revisited the experimental magnetic susceptibility and knight shift of four different compounds, La1x_{1-x}Srx_xCuO4_4, Bi2_2Sr2_2Ca1x_{1-x}Yx_xCu2_2O8_8, Bi2_2Sr2_2CaCu2_2O8+y_{8+y}, and YBa2_2Cu3_3O6+y_{6+y}, as a function of temperature and doping. The susceptibility can be described by the same function for all materials, having a magnetic and an electronic contributions. The former is the 2D antiferromagnetic (AF) square lattice response, with a characteristic temperature of magnetic correlations TmaxT_{max}. The latter is the `Pauli' term, revealing the gap opening in the electronic density of states at the pseudogap temperature TT^*. From precise fits of the data, we find that Tmax(p)T_{max}(p) decreases linearly as a function of doping (pp) over a wide range, but saturates abruptly in the overdoped regime. Concomitantly, T(p)T^*(p) is {\it linear and tangent} to the dome, either crossing or approaching Tmax(p)T_{max}(p) at the top of the dome, indicating a qualitative change of behavior from underdoped to overdoped regimes. Contrary to the idea that the pseudogap terminates just above optimal doping, our analysis suggests that the gap exists throughout the phase diagram. It is consistent with a pseudogap due to hole pairs, or `pairons', above TcT_c. We conclude that TmaxT_{max}, reflecting the AF magnetic correlations, has often been misinterpreted as the pseudogap temperature TT^*.

Keywords

Cite

@article{arxiv.2202.02589,
  title  = {Cuprates phase diagram deduced from magnetic susceptibility: what is the `true' pseudogap line?},
  author = {Yves Noat and Alain Mauger and Minoru Nohara and Hiroshi Eisaki and Shigeyuki Ishida and William Sacks},
  journal= {arXiv preprint arXiv:2202.02589},
  year   = {2022}
}

Comments

Solid State Communications (in press, February 2022)