English

Collective magnetic Higgs excitation in a pyrochlore ruthenate

Strongly Correlated Electrons 2023-08-15 v2 Materials Science

Abstract

The emergence of scalar Higgs-type amplitude modes in systems where symmetry is spontaneously broken has been a highly successful, paradigmatic description of phase transitions, with implications ranging from high-energy particle physics to low-energy condensed matter systems. Here, we uncover two successive high temperature phase transitions in the pyrochlore magnet Nd2_2Ru2_2O7_7 at TN=147T_{\mathrm{N}} = 147 K and T=97T^* = 97 K, that lead to giant phonon instabilities and culminate in the emergence of a highly coherent excitation. This coherent excitation, distinct from other phonons and from conventional magnetic modes, stabilizes at a low energy of 3 meV. We assign it to a collective Higgs-type amplitude mode, that involves bond energy modulations of the Ru4_4 tetrahedra. Its striking two-fold symmetry, incompatible with the underlying crystal structure, highlights the possibility of multiple entangled broken symmetries.

Keywords

Cite

@article{arxiv.2204.12124,
  title  = {Collective magnetic Higgs excitation in a pyrochlore ruthenate},
  author = {Dirk Wulferding and Junkyeong Kim and Mi Kyung Kim and Yang Yang and Jae Hyuck Lee and Dongjoon Song and Dongjin Oh and Heung-Sik Kim and Li Ern Chern and Yong Baek Kim and Minji Noh and Hyunyong Choi and Sungkyun Choi and Natalia B. Perkins and Changyoung Kim and Seung Ryong Park},
  journal= {arXiv preprint arXiv:2204.12124},
  year   = {2023}
}