English

Chiral Order and Multiferroic Domain Relaxation in NaFeGe$_2$O$_6$

Strongly Correlated Electrons 2021-11-17 v1

Abstract

The magnetic structure and the multiferroic relaxation dynamics of NaFeGe2_2O6_6 were studied by neutron scattering on single crystals partially utilizing polarization analysis. In addition to the previously reported transitions, the incommensurate spiral ordering of Fe3+^{3+} moments in the acac plane develops an additional component along the crystallographic bb direction below T5 KT\approx 5\text{ K}, which coincides with a lock-in of the incommensurate modulation. The quasistatic control of the spin-spiral handedness, respectively of the vector chirality, by external electric fields proves the invertibility of multiferroic domains down to the lowest temperature. Time-resolved measurements of the multiferroic domain inversion in NaFeGe2_2O6_6 reveal a simple temperature and electric-field dependence of the multiferroic relaxation that is well described by a combined Arrhenius-Merz relation, as it has been observed for TbMnO3_3. The maximum speed of domain wall motion is comparable to the spin wave velocity.

Keywords

Cite

@article{arxiv.2105.06875,
  title  = {Chiral Order and Multiferroic Domain Relaxation in NaFeGe$_2$O$_6$},
  author = {S. Biesenkamp and D. Gorkov and W. Schmidt and K. Schmalzl and Y. Sidis and P. Becker and L. Bohatý and M. Braden},
  journal= {arXiv preprint arXiv:2105.06875},
  year   = {2021}
}