English

Aromaticity in a Surface Deposited Cluster: Pd$_4$ on TiO$_2$ (110)

Materials Science 2012-04-12 v1

Abstract

We report the presence of \sigma-aromaticity in a surface deposited cluster, Pd4_4 on TiO2_2 (110). In the gas phase, Pd4_4 adopts a tetrahedral structure. However, surface binding promotes a flat, \sigma-aromatic cluster. This is the first time aromaticity is found in surface deposited clusters. Systems of this type emerge as a promising class of catalyst, and so realization of aromaticity in them may help to rationalize their reactivity and catalytic properties, as a function of cluster size and composition.

Keywords

Cite

@article{arxiv.1112.4032,
  title  = {Aromaticity in a Surface Deposited Cluster: Pd$_4$ on TiO$_2$ (110)},
  author = {Jin Zhang and Anastassia N. Alexandrova},
  journal= {arXiv preprint arXiv:1112.4032},
  year   = {2012}
}

Comments

4 pages, 3 figures