We report measurements of optical absorption in the zig-zag antiferromagnet α-RuCl3 as a function of temperature, T, magnetic field, B, and photon energy, ℏω in the range ∼ 0.3 to 8.3 meV, using time-domain terahertz spectroscopy. Polarized measurements show that 3-fold rotational symmetry is broken in the honeycomb plane from 2 K to 300 K. We find a sharp absorption peak at 2.56 meV upon cooling below the N\'eel temperature of 7 K at B=0 that we identify as magnetic-dipole excitation of a zero-wavevector magnon, or antiferromagnetic resonance (AFMR). With application of B, the AFMR broadens and shifts to lower frequency as long-range magnetic order is lost in a manner consistent with transitioning to a spin-disordered phase. From direct, internally calibrated measurement of the AFMR spectral weight, we place an upper bound on the contribution to the dc susceptibility from a magnetic excitation continuum.
@article{arxiv.1704.07357,
title = {Antiferromagnetic resonance and terahertz continuum in $\alpha-$RuCl$_3$},
author = {A. Little and Liang Wu and P. Lampen-Kelley and A. Banerjee and S. Patankar and D. Rees and C. A. Bridges and J. -Q. Yan and D. Mandrus and S. E. Nagler and J. Orenstein},
journal= {arXiv preprint arXiv:1704.07357},
year = {2017}
}
Comments
5 pages, 3 figures in the main text. To appear in Phys. Rev. Lett., magnetic field data included. Supplementary information also included