Time-Frequency Resolved Coherent Anti-Stokes Raman Scattering (TFRCARS) was recently proposed as a means to implement quantum logic using the molecular ro-vibrational manifold as a quantum register [R. Zadoyan et al., Chem. Phys. 266, 323 (2001)]. We give a concrete example of how this can be accomplished through an illustrative algorithm that solves the Deutsch-Jozsa problem. We use realistic molecular parameters to recognize that, as the problem size expands, shaped pulses must be tailored to maintain fidelity of the algorithm.
@article{arxiv.quant-ph/0110041,
title = {An Implementation of the Deutsch-Jozsa Algorithm on Molecular Vibronic Coherences Through Four-Wave Mixing: a Theoretical Study},
author = {Zsolt Bihary and David R. Glenn and Daniel A. Lidar and V. Ara Apkarian},
journal= {arXiv preprint arXiv:quant-ph/0110041},
year = {2016}
}
Comments
Replaced with published version. 14 pages, 2 figures, 1 table