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Molecular ro-vibronic coherences, joint energy-time distributions of quantum amplitudes, are selectively prepared, manipulated, and imaged in Time-Frequency-Resolved Coherent Anti-Stokes Raman Scattering (TFRCARS) measurements using…

Chemical Physics · Physics 2009-11-07 R. Zadoyan , D. Kohen , D. A. Lidar , V. A. Apkarian

A new approach to the implementation of a quantum computer by high-resolution nuclear magnetic resonance (NMR) is described. The key feature is that two or more line-selective radio-frequency pulses are applied simultaneously. A three-qubit…

Quantum Physics · Physics 2007-05-23 N Linden H Barjat R Freeman

For a practical quantum computer to operate, it will be essential to properly manage decoherence. One important technique for doing this is the use of "decoherence-free subspaces" (DFSs), which have recently been demonstrated. Here we…

Quantum Physics · Physics 2009-11-07 Masoud Mohseni , Jeffrey S. Lundeen , Kevin J. Resch , Aephraim M. Steinberg

We offer an improved method for using a nuclear-magnetic-resonance quantum computer (NMRQC) to solve the Deutsch-Jozsa problem. Two known obstacles to the application of the NMRQC are exponential diminishment of density-matrix elements with…

Quantum Physics · Physics 2009-11-06 John M. Myers , A. F. Fahmy , S. J. Glaser , R. Marx

The Deutsch-Jozsa algorithm is experimentally demonstrated for three-qubit functions using pure coherent superpositions of Li$_{2}$ rovibrational eigenstates. The function's character, either constant or balanced, is evaluated by first…

Quantum Physics · Physics 2009-11-07 Jiri Vala , Zohar Amitay , Bo Zhang , Stephen R. Leone , Ronnie Kosloff

Nuclear magnetic resonance (NMR) has been widely used as a demonstrative medium for showcasing the ability for quantum computations to outperform classical ones. A large number of such experiments performed have been implementations of the…

Emerging Technologies · Computer Science 2015-03-19 Alastair A. Abbott , Matthias Bechmann , Cristian S. Calude , Angelika Sebald

That superpositions of states can be useful for performing tasks in quantum systems has been known since the early days of quantum information, but only recently has quantitative theory of quantum coherence been proposed. Here we apply that…

Quantum Physics · Physics 2016-02-16 Mark Hillery

A chirped-pulse quantum control scheme applicable to Coherent Anti-Stokes Raman Scattering spectroscopy, named as C-CARS, is presented aimed at maximizing the vibrational coherence in molecules. It implies chirping of three incoming pulses…

Quantum Physics · Physics 2022-12-19 Jabir Chathanathil , Dmitry Budker , Svetlana A. Malinovskaya

Quantum computing implementations under consideration today typically deal with systems with microscopic degrees of freedom such as photons, ions, cold atoms, and superconducting circuits. The quantum information is stored typically in…

Quantum Physics · Physics 2016-05-04 Henry Semenenko , Tim Byrnes

The theory of stochastic processes impacts both physical and social sciences. At the molecular scale, stochastic dynamics is ubiquitous because of thermal fluctuations. The Fokker-Plank-Smoluchowski equation models the time evolution of the…

Single-shot time resolved Coherent Anti-Stokes Raman Scattering (CARS) is presented as a viable method for fast measurements of molecular spectra. The method is based on the short spatial extension of femtosecond pulses and maps time delays…

Optics · Physics 2009-11-13 Yuri Paskover , I. Sh. Averbukh , Yehiam Prior

We implemented the refined Deutsch-Jozsa algorithm on a 3-bit nuclear magnetic resonance quantum computer, which is the meaningful test of quantum parallelism because qubits are entangled. All of the balanced and constant functions were…

Quantum Physics · Physics 2009-10-31 Jaehyun Kim , Jae-Seung Lee , Soonchil Lee , Chaejoon Cheong

A detailed description of the development of a three qubit NMR realization of the Deutsch-Jozsa algorithm [Collins et.al., Phys. Rev. A 62, 022304 (2000)] is provided. The theoretical and experimental techniques used for the reduction of…

Quantum Physics · Physics 2007-05-23 David Collins , K. W. Kim , W. C. Holton , H. Sierzputowska-Gracz , E. O. Stejskal

We discuss the ensemble version of the Deutsch-Jozsa (DJ) algorithm which attempts to provide a "scalable" implementation on an expectation-value NMR quantum computer. We show that this ensemble implementation of the DJ algorithm is at best…

Quantum Physics · Physics 2016-09-08 Arvind , David Collins

We propose a physical scheme for implementing the Deutsch-Jozsa algorithm using atomic ensembles and optical devices. The scheme has inherent fault tolerance to the realistic noise and efficient scaling with the number of ensembles for some…

Quantum Physics · Physics 2007-05-23 Ping Dong , Zheng-Yuan Xue , Ming Yang , Zhuo-Liang Cao

We compare the Frequency-Resolved Frozen Phonon Multislice (FRFPMS) method, introduced in Phys. Rev. Lett. 124, 025501 (2020), with other theoretical approaches used to account for the inelastic scattering of high energy electrons, namely…

Materials Science · Physics 2023-04-27 Paul M. Zeiger , Juri Barthel , Leslie J. Allen , Ján Rusz

Coherent Raman scattering spectroscopy is studied purposely, with the Gaussian ultrashort pulses as a hands-on elucidatory extraction tool of the clean coherent Raman resonant spectra from the overall measured data contaminated with the…

Optics · Physics 2017-04-05 Gombojav O. Ariunbold , Narangerel Altangerel

Practical implementation of many quantum algorithms known today is limited by the coherence time of the executing quantum hardware and quantum sampling noise. Here we present a machine learning algorithm, NISQRC, for qubit-based quantum…

Spontaneous vibrational Raman scattering is a ubiquitous form of light-matter interaction whose description necessitates quantization of the electromagnetic field. It is usually considered as an incoherent process because the scattered…

Quantum Physics · Physics 2023-07-18 Valeria Vento , Santiago Tarrago Velez , Anna Pogrebna , Christophe Galland

We present a novel approach to quantum algorithms, by taking advantage of modular values, i.e., complex and unbounded quantities resulting from specific post-selected measurement scenarios. Our focus is on the problem of ascertaining…

Quantum Physics · Physics 2024-06-12 Lorena Ballesteros Ferraz , Timoteo Carletti , Yves Caudano
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