Vacancy-induced spin textures and their interactions in a classical spin liquid
Abstract
Motivated by experiments on the archetypal frustrated magnet SrCrGaO (SCGO), we study the classical Heisenberg model on the pyrochlore slab (Kagom\'e bilayer) lattice with site-dilution . This allows us to address generic aspects of the physics of non-magnetic vacancies in a classical spin liquid. We explicitly demonstrate that the pure () system remains a spin-liquid down to the lowest temperatures, with an unusual {\em non-monotonic} temperature dependence of the susceptibility, which even turns diamagnetic for the apical spins between the two kagome layers. For but small, the low temperature magnetic response of the system is most naturally described in terms of the properties of spatially extended spin textures that cloak an "orphan" Cr spin in direct proximity to a pair of missing sites belonging to the same triangular simplex. In the limit, these orphan-texture complexes each carry a net magnetization that is exactly half the magnetic moment of an individual spin of the undiluted system. Furthermore, we demonstrate that they interact via an entropic {\em temperature dependent} {\em pair-wise exchange interaction} that has a logarithmic form at short-distances and decays exponentially beyond a thermal correlation length . The sign of depends on whether the two orphan spins belong to the same Kagome layer or not. We provide a detailed analytical account of these properties using an effective field theory approach specifically tailored for the problem at hand. These results are in quantitative agreement with large-scale Monte Carlo numerics.
Cite
@article{arxiv.1204.4970,
title = {Vacancy-induced spin textures and their interactions in a classical spin liquid},
author = {Arnab Sen and Kedar Damle and R. Moessner},
journal= {arXiv preprint arXiv:1204.4970},
year = {2015}
}
Comments
two-column PRB format; 21 pages; 14 .eps figures. v2: a minor typo fixed