English

Vacancy-induced spin textures and their interactions in a classical spin liquid

Strongly Correlated Electrons 2015-06-04 v2

Abstract

Motivated by experiments on the archetypal frustrated magnet SrCr9p_{9p}Ga129p_{12-9p}O19_{19} (SCGO), we study the classical Heisenberg model on the pyrochlore slab (Kagom\'e bilayer) lattice with site-dilution x=1px=1-p. This allows us to address generic aspects of the physics of non-magnetic vacancies in a classical spin liquid. We explicitly demonstrate that the pure (x=0x=0) system remains a spin-liquid down to the lowest temperatures, with an unusual {\em non-monotonic} temperature dependence of the susceptibility, which even turns diamagnetic for the apical spins between the two kagome layers. For x>0x> 0 but small, the low temperature magnetic response of the system is most naturally described in terms of the properties of spatially extended spin textures that cloak an "orphan" S=3/2S=3/2 Cr3+^{3+} spin in direct proximity to a pair of missing sites belonging to the same triangular simplex. In the T0T \rightarrow 0 limit, these orphan-texture complexes each carry a net magnetization that is exactly half the magnetic moment of an individual spin of the undiluted system. Furthermore, we demonstrate that they interact via an entropic {\em temperature dependent} {\em pair-wise exchange interaction} Jeff(T,r)TJ(rT)J_{eff}(T,\vec{r}) \sim T {\mathcal J} (\vec{r} \sqrt{T}) that has a logarithmic form at short-distances and decays exponentially beyond a thermal correlation length ξ(T)1/T\xi(T) \sim 1/\sqrt{T}. The sign of JeffJ_{eff} depends on whether the two orphan spins belong to the same Kagome layer or not. We provide a detailed analytical account of these properties using an effective field theory approach specifically tailored for the problem at hand. These results are in quantitative agreement with large-scale Monte Carlo numerics.

Keywords

Cite

@article{arxiv.1204.4970,
  title  = {Vacancy-induced spin textures and their interactions in a classical spin liquid},
  author = {Arnab Sen and Kedar Damle and R. Moessner},
  journal= {arXiv preprint arXiv:1204.4970},
  year   = {2015}
}

Comments

two-column PRB format; 21 pages; 14 .eps figures. v2: a minor typo fixed

R2 v1 2026-06-21T20:53:18.027Z