English

Ultra-long-range dynamic correlations in a microscopic model for aging gels

Soft Condensed Matter 2017-06-21 v1

Abstract

We use large-scale computer simulations to explore the non-equilibrium aging dynamics in a microscopic model for colloidal gels. We find that gelation resulting from a kinetically-arrested phase separation is accompanied by `anomalous' particle dynamics revealed by superdiffusive particle motion and compressed exponential relaxation of time correlation functions. Spatio-temporal analysis of the dynamics reveals intermittent heterogeneities producing spatial correlations over extremely large length scales. Our study is the first microscopically-resolved model reproducing all features of the spontaneous aging dynamics observed experimentally in soft materials.

Keywords

Cite

@article{arxiv.1605.09770,
  title  = {Ultra-long-range dynamic correlations in a microscopic model for aging gels},
  author = {Pinaki Chaudhuri and Ludovic Berthier},
  journal= {arXiv preprint arXiv:1605.09770},
  year   = {2017}
}
R2 v1 2026-06-22T14:14:10.704Z