Moir{\'e} heterostructures, created by stacking two-dimensional (2D) materials together with a finite lattice mismatch or rotational twist, represent a new frontier of designer quantum materials. Typically, however, this requires the painstaking manual assembly of heterostructures formed from exfoliated materials. Here, we observe clear spectroscopic signatures of moir{\'e} lattice formation in epitaxial heterostructures of monolayer (ML) NbSe2 grown on graphite substrates. Our angle-resolved photoemission measurements and theoretical calculations of the resulting electronic structure reveal moir{\'e} replicas of the graphite π states forming pairs of interlocking Dirac cones. Interestingly, these intersect the NbSe2 Fermi surface at the k-space locations where NbSe2's charge-density wave (CDW) gap is maximal in the bulk. This provides a natural route to understand the lack of CDW enhancement for ML-NbSe2/graphene as compared to a more than four-fold enhancement for NbSe2 on insulating support substrates, and opens new prospects for using moir{\'e} engineering for controlling the collective states of 2D materials.
@article{arxiv.2506.00449,
title = {Resonant interlayer coupling in NbSe$_2$-graphite epitaxial moir{\'e} superlattices},
author = {S. Mo and K. Kovalenka and S. Buchberger and B. K. Saika and A. Azhar and A. Rajan and A. Zivanovic and Y. -C. Yao and R. V. Belosludov and M. D. Watson and M. S. Bahramy and P. D. C. King},
journal= {arXiv preprint arXiv:2506.00449},
year = {2026}
}
Comments
11 pages including supplementary information, 4+5 figures