English

Mechanochemical feedback drives complex inertial dynamics in active solids

Soft Condensed Matter 2025-12-29 v2 Materials Science Statistical Mechanics Chaotic Dynamics

Abstract

Active solids combine internal active driving with elasticity to realize states with nonequilibrium mechanics and autonomous motion. They are often studied in overdamped settings, e.g., in soft materials, and the role of inertia is less explored. We construct a model of a chemically active solid that incorporates mechanochemical feedback and show that, when feedback overwhelms mechanical damping, autonomous inertial dynamics can spontaneously emerge through sustained consumption of chemical fuel. By combining numerical simulations, analysis and dynamical systems approaches, we show how active feedback drives complex nonlinear dynamics on multiple time-scales, including limit cycles and chaos. Our results suggest design principles for creating ultrafast actuators and autonomous machines from soft, chemically-powered solids.

Keywords

Cite

@article{arxiv.2505.18272,
  title  = {Mechanochemical feedback drives complex inertial dynamics in active solids},
  author = {Siddhartha Sarkar and Biswarup Ash and Yueyang Wu and Nicholas Boechler and Suraj Shankar and Xiaoming Mao},
  journal= {arXiv preprint arXiv:2505.18272},
  year   = {2025}
}

Comments

7 pages, 4 figures, SI included as ancillary file. Final published version with experimental parameters included

R2 v1 2026-07-01T02:34:43.767Z