English

Long-lived quantum coherent dynamics of a $\Lambda$-system driven by a thermal environment

Quantum Physics 2022-10-18 v2 Atomic Physics Chemical Physics

Abstract

We present a theoretical study of quantum coherent dynamics of a three-level Λ\Lambda system driven by a thermal environment (such as blackbody radiation), which serves as an essential building block of photosynthetic light-harvesting models and quantum heat engines. By solving the nonsecular Bloch-Redfield master equations, we obtain analytical results for the ground-state population and coherence dynamics and classify the dynamical regimes of the incoherently driven Λ\Lambda-system as underdamped and overdamped depending on whether the ratio Δ/[rf(p)]\Delta/[r f(p)] is greater or less than one, where Δ\Delta is the ground-state energy splitting, rr is the incoherent pumping rate, and f(p)f(p) is a function of the transition dipole alignment parameter pp. In the underdamped regime, we observe long-lived coherent dynamics that lasts for τc1/r\tau_c\simeq 1/r, even though the initial state of the Λ\Lambda-system contains no coherences in the energy basis. In the overdamped regime for p=1p = 1, we observe the emergence of coherent quasi-steady states with the lifetime τc=1.34(r/Δ2)\tau_{c} = 1.34 (r/\Delta^{2}), which have low von Neumann entropy compared to the conventional thermal states. We propose an experimental scenario for observing noise-induced coherent dynamics in metastable He^* atoms driven by x-polarized incoherent light. Our results suggest that thermal excitations can generate experimentally observable long-lived quantum coherent dynamics in the ground-state subspace of atomic and molecular Λ\Lambda systems in the absence of coherent driving.

Keywords

Cite

@article{arxiv.2108.07457,
  title  = {Long-lived quantum coherent dynamics of a $\Lambda$-system driven by a thermal environment},
  author = {Suyesh Koyu and Timur V. Tscherbul},
  journal= {arXiv preprint arXiv:2108.07457},
  year   = {2022}
}
R2 v1 2026-06-24T05:10:37.995Z