English

Improved Optimization for the Neural-network Quantum States and Tests on the Chromium Dimer

Chemical Physics 2024-09-24 v3 Quantum Physics

Abstract

The advent of Neural-network Quantum States (NQS) has significantly advanced wave function ansatz research, sparking a resurgence in orbital space variational Monte Carlo (VMC) exploration. This work introduces three algorithmic enhancements to reduce computational demands of VMC optimization using NQS: an adaptive learning rate algorithm, constrained optimization, and block optimization. We evaluate the refined algorithm on complex multireference bond stretches of H2O\rm H_2O and N2\rm N_2 within the cc-pVDZ basis set and calculate the ground-state energy of the strongly correlated chromium dimer (Cr2\rm Cr_2) in the Ahlrichs SV basis set. Our results achieve superior accuracy compared to coupled cluster theory at a relatively modest CPU cost. This work demonstrates how to enhance optimization efficiency and robustness using these strategies, opening a new path to optimize large-scale Restricted Boltzmann Machine (RBM)-based NQS more effectively and marking a substantial advancement in NQS's practical quantum chemistry applications.

Keywords

Cite

@article{arxiv.2404.09280,
  title  = {Improved Optimization for the Neural-network Quantum States and Tests on the Chromium Dimer},
  author = {Xiang Li and Jia-Cheng Huang and Guang-Ze Zhang and Hao-En Li and Zhu-Ping Shen and Chen Zhao and Jun Li and Han-Shi Hu},
  journal= {arXiv preprint arXiv:2404.09280},
  year   = {2024}
}

Comments

13 pages, 9 figures, and 2 tables

R2 v1 2026-06-28T15:53:47.208Z