The formation of flat electronic bands from long-wavelength superperiodic moir\'e potentials in van der Waals heterostructures underpins the creation and control of a host of highly-tuneable correlated and topological phases. The underlying moir\'e periodicity is, however, typically considered a fixed property of the heterostructure. Here, we show how the development of a charge-density wave (CDW) in one of the constituent materials can create an emergent moir\'e periodicity, realising a superperiodic potential in TiSe2/graphite epitaxial heterostructures with an order-of-magnitude longer wavelength than that expected from the normal-state lattice mismatch. We demonstrate how this drives the formation of a remarkably strong band flattening, which can be readily deactivated by carrier doping across the CDW phase transition, opening new prospects for engineering moir\'e matter by exploiting the rich many-body states of the parent compounds of 2D heterostructures.
@article{arxiv.2511.05648,
title = {Flat electronic bands from cooperative moir\'e and charge order},
author = {B. K. Saika and S. Buchberger and S. Mo and A. Rajan and D. Halliday and Y. -C. Yao and L. C. Rhodes and B. Sarpi and T. Balasubramanian and C. Polley and P. Wahl and P. D. C. King},
journal= {arXiv preprint arXiv:2511.05648},
year = {2025}
}
Comments
15 pages including supplementary information, 4+4 figures