English

Coupling interlayer excitons to whispering gallery modes in van der Waals heterostructures

Materials Science 2020-08-20 v2

Abstract

Van der Waals heterostructures assembled from two-dimensional materials offer a promising platform to engineer structures with desired optoelectronic characteristics. Here we use waveguide-coupled disk resonators made of hexagonal boron nitride (h-BN) to demonstrate cavity-coupled emission from interlayer excitons of a heterobilayer of two monolayer transition metal dichalcogonides. We sandwich a MoSe2_{\rm 2} - WSe2_{\rm 2} heterobilayer between two slabs of h-BN and directly pattern the resulting stack into waveguide-coupled disk resonators. This enables us to position the active materials into regions of highest optical field intensity, thereby maximizing the mode overlap and the coupling strength. Since the interlayer exciton emission energy is lower than the optical band gaps of the individual monolayers and since the interlayer transition itself has a weak oscillator strength, the circulating light is only weakly reabsorbed, which results in an unaffected quality factor. Our devices are fully waveguide-coupled and represent a promising platform for on-chip van der Waals photonics.

Keywords

Cite

@article{arxiv.2007.04886,
  title  = {Coupling interlayer excitons to whispering gallery modes in van der Waals heterostructures},
  author = {Ronja Khelifa and Patrick Back and Nikolaus Flöry and Shadi Nashashibi and Konstantin Malchow and Takashi Taniguchi and Kenji Watanabe and Achint Jain and Lukas Novotny},
  journal= {arXiv preprint arXiv:2007.04886},
  year   = {2020}
}

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Supplementary information included

R2 v1 2026-06-23T16:59:22.208Z