English

Comparison between exact and semilocal exchange potentials: An all-electron study for solids

Strongly Correlated Electrons 2016-08-07 v1 Materials Science

Abstract

The exact-exchange (EXX) potential, which is obtained by solving the optimized-effective potential (OEP) equation, is compared to various approximate semilocal exchange potentials for a set of selected solids (C, Si, BN, MgO, Cu2_{2}O, and NiO). This is done in the framework of the linearized augmented plane-wave method, which allows for a very accurate all-electron solution of electronic structure problems in solids. In order to assess the ability of the semilocal potentials to approximate the EXX-OEP, we considered the EXX total energy, electronic structure, electric-field gradient, and magnetic moment. An attempt to parameterize a semilocal exchange potential is also reported.

Keywords

Cite

@article{arxiv.1501.07105,
  title  = {Comparison between exact and semilocal exchange potentials: An all-electron study for solids},
  author = {Fabien Tran and Markus Betzinger and Peter Blaha and Stefan Blügel},
  journal= {arXiv preprint arXiv:1501.07105},
  year   = {2016}
}
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