English

Calculating the spin memory loss at Cu$|$metal interfaces from first principles

Materials Science 2022-07-07 v1 Mesoscale and Nanoscale Physics

Abstract

The role played by interfaces in metallic multilayers is not only to change the momenta of incident electrons; their symmetry lowering also results in an enhancement of the effects of spin-orbit coupling, in particular the flipping of the spins of conduction electrons. This leads to a significant reduction of a spin current through a metallic interface that is quantitatively characterized by a dimensionless parameter δ\delta called the spin memory loss (SML) parameter, the interface counterpart of the spin-flip diffusion length for bulk metals. In this paper we use first-principles scattering calculations that include temperature-induced lattice and spin disorder to systematically study three parameters that govern spin transport through metallic interfaces of Cu with Pt, Pd, Py (permalloy) and Co: the interface resistance, spin polarization and the SML. The value of δ\delta for a Cu|Pt interface is found to be comparable to what we recently reported for a Au|Pt interface [Gupta {\it et al.}, Phys. Rev. Lett. 124, 087702 (2020)]. For Cu|Py and Cu|Co interfaces, δ\delta decreases monotonically with increasing temperature to become negligibly small at room temperature. The calculated results are in good agreement with currently available experimental values in the literature. Inserting a Cu layer between Pt and the Py or Co layers slightly increases the total spin current dissipation at these "compound" interfaces.

Cite

@article{arxiv.2207.02395,
  title  = {Calculating the spin memory loss at Cu$|$metal interfaces from first principles},
  author = {Ruixi Liu and Kriti Gupta and Zhe Yuan and Paul J. Kelly},
  journal= {arXiv preprint arXiv:2207.02395},
  year   = {2022}
}
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