English

Atomic carbon chains as spin-transmitters: an \textit{Ab initio} transport study

Mesoscale and Nanoscale Physics 2015-05-14 v2

Abstract

An atomic carbon chain joining two graphene flakes was recently realized in a ground-breaking experiment by Jin {\it et al.}, Phys. Rev. Lett. {\bf 102}, 205501 (2009). We present {\it ab initio} results for the electron transport properties of such chains and demonstrate complete spin-polarization of the transmission in large energy ranges. The effect is due to the spin-polarized zig-zag edge terminating each graphene flake causing a spin-splitting of the graphene πz\pi_z bands, and the chain states. Transmission occurs when the graphene π\pi-states resonate with similar states in the strongly hybridized edges and chain. This effect should in general hold for any π\pi-conjugated molecules bridging the zig-zag edges of graphene electrodes. The polarization of the transmission can be controlled by chemically or mechanically modifying the molecule, or by applying an electrical gate.

Keywords

Cite

@article{arxiv.0909.1756,
  title  = {Atomic carbon chains as spin-transmitters: an \textit{Ab initio} transport study},
  author = {Joachim A. Fuerst and Mads Brandbyge and Antti-Pekka Jauho},
  journal= {arXiv preprint arXiv:0909.1756},
  year   = {2015}
}
R2 v1 2026-06-21T13:44:30.571Z