Anomalous Relativistic Emission from Self-Modulated Plasma Mirrors

The interaction of intense laser pulses with plasma mirrors has demonstrated the ability to generate high-order harmonics, producing a bright source of extreme ultraviolet (XUV) radiation and attosecond pulses. Here, we report an unexpected transition in this process. We show that the loss of spatio-temporal coherence in the reflected high-harmonics can lead to a new regime of highly-efficient coherent XUV generation, with an extraordinary property where the radiation is directionally anomalous, propagating parallel to the mirror surface. With analytical calculations and numerical particle-in-cell simulations, we discover that the radiation emission is due to laser-driven oscillations of relativistic electron nanobunches which originate from a plasma surface instability induced by collisionless absorption of the laser.