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We find that a donor-doped band-gap material can enhance the overall high-order harmonic generation (HHG) efficiency by several orders of magnitude, compared with undoped and acceptor-doped materials. This significant enhancement, predicted…

Optics · Physics 2019-01-30 Chuan Yu , Kenneth K. Hansen , Lars Bojer Madsen

The potential for low-threshold optical nonlinearity has received significant attention in the fields of photonics and conceptual optical neuron networks. Excitons in two-dimensional (2D) semiconductors are particularly promising in this…

The strong-field induced generation of nonclassical states of light is not only a subject of fundamental research but also has potential usage in quantum information science and technology. The emerging field of strong-field quantum optics…

Quantum Physics · Physics 2025-03-21 Christian Saugbjerg Lange , Thomas Hansen , Lars Bojer Madsen

Nonlinear optical phenomena are widely used for the study of semiconductor materials. The paper presents an overview of experimental and theoretical studies of excitons by the method of optical second and third harmonics generation in…

Materials Science · Physics 2018-08-29 D. R. Yakovlev , V. V. Pavlov , A. V. Rodina , R. V. Pisarev , J. Mund , W. Warkentin , M. Bayer

The recombination of electron-hole pairs injected in extended conjugated systems is modeled as a multi-pathway vibron-driven relaxation in monoexcited state-space. The computed triplet-to-singlet ratio of exciton formation times $r =…

Materials Science · Physics 2009-11-07 Stoyan Karabunarliev , Eric. R. Bittner

We report strong third-harmonic generation (THG) in monolayer graphene grown by chemical vapor deposition (CVD) and transferred to an amorphous silica (glass) substrate; the photon energy is in three-photon resonance with the…

Mesoscale and Nanoscale Physics · Physics 2013-06-12 Sung-Young Hong , Jerry I. Dadap , Nicholas Petrone , Po-Chun Yeh , James Hone , Richard M. Osgood

We explore the roles of electronic band structure and Coulomb interactions in solid-state HHG by studying the optical response of linear atomic chains and carbon nanotubes to intense ultrashort pulses. Specifically, we simulate electron…

Mesoscale and Nanoscale Physics · Physics 2020-03-18 Sandra de Vega , Joel D. Cox , Fernando Sols , F. Javier García de Abajo

Second-order nonlinear optical interactions such as sum- and difference-frequency generation are widely used for bioimaging and as selective probes of interfacial environments. However, inefficient nonlinear optical conversion often leads…

Optics · Physics 2015-05-07 Aaron J. Goodman , William A. Tisdale

A theory for laser-driven electron dynamics and high-harmonic generation in bulk solids with two lattice sites per unit cell of arbitrary dimension is formulated. In tight-binding approximation, such solids can be described by $2\times 2$…

Mesoscale and Nanoscale Physics · Physics 2024-03-12 Daniel Moos , Hannah Jürß , Dieter Bauer

We develop a general theory of electron--hole recombination in organic light emitting diodes that leads to formation of emissive singlet excitons and nonemissive triplet excitons. We briefly review other existing theories and show how our…

Materials Science · Physics 2009-11-07 K. Tandon , S. Ramasesha , S. Mazumdar

We study high-harmonic generation (HHG) in the one-dimensional Hubbard model in order to understand its relation to elementary excitations as well as the similarities and differences to semiconductors. The simulations are based on the…

Strongly Correlated Electrons · Physics 2021-01-13 Yuta Murakami , Shintaro Takayoshi , Akihisa Koga , Philipp Werner

The study of the non-linear response of matter to high electric fields has recently encompassed harmonic generation in solids at near-infrared (NIR) driving wavelengths. Interest has been driven by the prospect of ultrafast signal…

Organic cavity polaritons are bosonic quasi-particles that arise from the strong interaction between organic molecular excitons and photons within microcavities. The spectral dispersion of third harmonic generation near resonance with the…

Optics · Physics 2018-10-08 Bin Liu , Michael Crescimanno , Robert J. Twieg , Kenneth D. Singer

We report on theoretical study of second-harmonic generation (SHG) in plasmonic nanostructures interacting with two-level quantum emitters (QE) under incoherent energy pump. We generalize driven-dissipative Tavis-Cummings model by…

Optics · Physics 2021-03-17 Maxim Sukharev , Oleksiy Roslyak , Andrei Piryatinski

We investigate the Hall effect in two different theoretical models of strongly correlated systems: a system made of weakly coupled Luttinger liquids, in the presence of umklapp scattering, and the 2D triangular lattice, with…

Strongly Correlated Electrons · Physics 2008-12-11 Gladys León

The strong-field process of high-harmonic generation (HHG) has, in recent years, been treated from a quantum optical perspective in the emerging research area of strong-field quantum optics. These investigations show that HHG radiation is,…

Quantum Physics · Physics 2026-02-19 Christian Saugbjerg Lange , Lars Bojer Madsen

Higgs spectroscopy is a new field in which Higgs modes in nonequilibrium superconductors are analyzed to gain information about the ground state. One experimental setup in which the Higgs mode in s-wave superconductors was observed is…

Superconductivity · Physics 2020-05-26 Lukas Schwarz , Dirk Manske

Electronic correlations arise from the competition between the electrons' kinetic and Coulomb interaction energy and give rise to a rich phase diagram and many emergent quasiparticles. The binding of doubly-occupied and empty sites into a…

Strongly Correlated Electrons · Physics 2024-09-10 Edin Kapetanović , Guglielmo Nicola Gigante , Malte Schüler , Tim O. Wehling , Erik van Loon

The optical conductivity of a polaronic charge carrier in the intermediate and strong-coupling regimes is calculated for a tight-binding electron using exact diagonalization. Two different simple models of the electron-phonon coupling are…

Condensed Matter · Physics 2007-05-23 M. Capone , W. Stephan

High-order harmonic responses from three $C_{20}$ isomers: fullerene, ring, and bowl, are calculated within the modified Lewenstein model for molecular systems. Spectra for all three structures exhibit intense modulations of the harmonic…

Quantum Physics · Physics 2022-03-31 F. Cajiao - Vélez , A. Jaron