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Raman scattering excitation (RSE) is an experimental technique in which the spectrum is made up by sweeping the excitation energy when the detection energy is fixed. We study the low-temperature ($T$=5~K) RSE spectra measured on four high…

We simulate a third-order nonlinear signal in a pump-probe spectroscopy from the interference between first- and second-order wavepackets (WPs), as well as from a state-to-state transition for Stokes and coherent anti-Stokes pathways in the…

Chemical Physics · Physics 2026-04-14 Subho Mitra , Arijit K. De

Stimulated Raman scattering (SRS) in plasma in the degenerate regime is studied theoretically and numerically. Different from normal SRS with the non-degenerate eigen electrostatic mode excited, the degenerate SRS is developed at plasma…

Plasma Physics · Physics 2022-03-25 Yao Zhao , Suming Weng , Zhengming Sheng , Jianqiang Zhu

In its usual implementation, the Raman amplifier features only one pump carrier frequency. However, pulses with well-separated frequencies can also be Raman amplified while compressed in time. Amplification with frequency-separated pumps is…

Plasma Physics · Physics 2018-04-04 Ido Barth , Nathaniel J. Fisch

Plasma is capable of mediating the conversion of two pump photons into two different photons through a relativistic four-wave mixing nonlinearity. Spontaneously created photon pairs are emitted at symmetric angles with respect to the…

Plasma Physics · Physics 2025-01-07 Kenan Qu , Nathaniel J. Fisch

Strongly coupled large-angle stimulated Raman scattering (LA SRS) of a short intense laser pulse proceeds in a plane plasma-filled capillary differently than in a plasma with open boundaries. Oblique mirror reflections off capillary walls…

Plasma Physics · Physics 2009-11-10 Serguei Kalmykov , Patrick Mora

We consider a long fiber-optical link consisting of alternating dispersive and nonlinear segments, i.e., a split-step model (SSM), in which the dispersion and nonlinearity are completely separated. Passage of a soliton through one cell of…

Pattern Formation and Solitons · Physics 2007-05-23 Rodislav Driben , Boris A. Malomed

In a recent experiment (N. Wagner et al., PNAS v103, p13279) on SF$_{6}$, a high-harmonic generating laser pulse is preceded by a pump pulse which stimulates Raman-active modes in the molecule. Varying the time delay between the two pulses…

Atomic Physics · Physics 2009-11-13 Zachary B. Walters , Stefano Tonzani , Chris H. Greene

A coherent microwave radiation, concomitant with experiments of stimulated Raman scattering (SRS) in weakly compressed hydrogen, had been observed; qualitative and quantitative results had been obtained, and are given in this article. .An…

Optics · Physics 2007-05-23 Boris Oksengorn

Recently, the verification of stimulated Raman side-scattering (SRSS) in different laser inertial confinement fusion ignition schemes poses an underlying risk of SRSS on ignition. In this paper, we propose a method to use the non-uniform…

Plasma Physics · Physics 2023-05-12 Xiaobao Jia , Qing Jia , Rui Yan , Jian Zheng

The hybrid Stimulated Raman Scattering - Two Plasmon Decay instability had shown to play the dominant role for plasma waves excitation and energy absorption at interaction of very intense femtosecond obliquely incident $p$-polarized laser…

Plasma Physics · Physics 2021-01-04 I. Tsymbalov , D. Gorlova , A. Savel'ev

We demonstrate the acquisition of stimulated Raman scattering spectra with the use of a single femtosecond pulse. High resolution vibrational spectra are obtained by shifting the phase of a narrow band of frequencies in the broadband input…

Optics · Physics 2015-05-20 Hadas Frostig , Ori Katz , Adi Natan , Yaron Silberberg

Quantum logic gates performed via two-photon stimulated-Raman transitions in ions and atoms are fundamentally limited by spontaneous scattering errors. Recent theoretical treatment of these scattering processes has predicted no lower bound…

As a highly sensitive vibrational imaging method, stimulated Raman scattering (SRS) microscopy is finding various applications, while its theoretical treatment seems still under development. Here we present a theoretical estimation of…

Optics · Physics 2024-03-11 Yasuyuki Ozeki

Stationary light pulses (SLPs), i.e., light pulses without motion, are formed via the retrieval of stored probe pulses with two counter-propagating coupling fields. We show that there exist non-negligible hybrid Raman excitations in media…

Raman-based technologies have enabled many ground-breaking scientific discoveries related to surface science, single molecule chemistry and biology. For example, researchers have identified surface bound molecules by their Raman vibrational…

Optics · Physics 2020-03-12 Xiaoqin Shen , Hyungwoo Choi , Dongyu Chen , Wei Zhao , Andrea M. Armani

Raman scattering from the out-of-plane vibrational modes (A$_{1\text{g}}$/A'$_{1}$), which originate from the bulk-inactive out-of-plane B$^{1}_{2\text{g}}$ mode, are studied in few-layer MoTe$_{2}$. Temperature-dependent measurements…

Due to their high circulating intensities, ultra-high quality factor dielectric whispering-gallery mode resonators have enabled the development of low threshold Raman microlasers. Subsequently, other Raman-related phenomena, such as…

By using spontaneous Raman processes in the high gain regime, we produce two independent Raman Stokes fields from an atomic ensemble. Temporal beating is observed between the two directly generated Stokes fields in a single realization. The…

Quantum Physics · Physics 2010-05-27 Li-Qing Chen , Cheng-ling Bian , Guo-Wan Zhang , Z. Y. Ou , Weiping Zhang

We numerically study Stokes beam generation in an array of discrete waveguides. The feasibility of generation and steering of spatial solitons due to nonlinear Raman response is demonstrated for the first time

Pattern Formation and Solitons · Physics 2007-05-23 Clark A. Merchant , Igor V. Mel'nikov , J. Stewart Aitchison