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The ability to design quantum systems that decouple from environmental noise sources is highly desirable for development of quantum technologies with optimal coherence. The chemical tunability of electronic states in magnetic molecules…

Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…

Quantum Physics · Physics 2022-11-11 Alexander A. Wood , Russell M. Goldblatt , Robert E. Scholten , Andy M. Martin

Applications of quantum simulation algorithms to obtain electronic energies of molecules on noisy intermediate-scale quantum (NISQ) devices require careful consideration of resources describing the complex electron correlation effects. In…

Quantum Physics · Physics 2020-04-17 Mekena Metcalf , Nicholas P. Bauman , Karol Kowalski , Wibe A. de Jong

A solid-state implementation of a quantum computer composed entirely of silicon is proposed. Qubits are Si-29 nuclear spins arranged as chains in a Si-28 (spin-0) matrix with Larmor frequencies separated by a large magnetic field gradient.…

Quantum Physics · Physics 2007-05-23 T. D. Ladd , J. R. Goldman , F. Yamaguchi , Y. Yamamoto , E. Abe , K. M. Itoh

It is predicted that nuclear spin conversion in molecules can be efficiently controlled by strong laser radiation resonant to rovibrational molecular transition. The phenomenon can be used for substantial enrichment of spin isomers, or for…

Chemical Physics · Physics 2009-11-06 P. L. Chapovsky

Optically addressable molecular triplet spins provide a chemically tunable platform for quantum application, but their coherence is often limited by interactions with surrounding spin baths. Here we demonstrate controlled suppression of…

Molecular spins offer promise in emerging quantum technologies such as quantum sensing and computing. At low temperatures, nuclear spin-spin interactions affect electron spin coherence lifetimes through pure dephasing. Nuclear-spin noise…

Quantum Physics · Physics 2026-05-06 Timothy J. Krogmeier , James Bradley , Anthony W. Schlimgen , Kade Head-Marsden

We theoretically analyze the performance of the nuclear magnetic resonance (NMR) spectroscopy with a superconducting flux qubit (FQ). Such NMR with the FQ is attractive because of the possibility to detect the relatively small number of…

Neuromorphic computing approaches become increasingly important as we address future needs for efficiently processing massive amounts of data. The unique attributes of quantum materials can help address these needs by enabling new…

Nuclear magnetic resonance spectroscopy with solid-state spin sensors is a promising pathway for the detection of nuclear spins at the micro- and nanoscale. Although many nanoscale experiments rely on a single sensor spin for the detection…

Nuclear magnetic resonance (NMR) schemes can be applied to micron-, and nanometer-sized samples by the aid of quantum sensors such as nitrogen-vacancy (NV) color centers in diamond. These minute devices allow for magnetometry of nuclear…

Quantum Physics · Physics 2021-07-19 C. Munuera-Javaloy , R. Puebla , J. Casanova

The procedure for simulating the nuclear magnetic resonance spectrum linked to the spin system of a molecule for a certain nucleus entails diagonalizing the associated Hamiltonian matrix. As the dimensions of said matrix grow exponentially…

Quantum Physics · Physics 2024-10-29 Joaquín Ossorio-Castillo , Alexandre Rodríguez-Coello

Algorithmic Cooling is a method that uses novel data compression techniques and simplecquantum computing devices to improve NMR spectroscopy, and to offer scalable NMR quantum computers. The algorithm recursively employs two steps. A…

Quantum Physics · Physics 2009-11-11 Jose M. Fernandez , Tal Mor , Yossi Weinstein

Reservoir computing with optical devices offers an energy-efficient approach for time-series forecasting. Quantum dot lasers with feedback are modelled in this paper to explore the extent to which increased complexity in the charge carrier…

Computational Physics · Physics 2024-11-05 Huifang Dong , Lina Jaurigue , Kathy Lüdge

Quantum information processing is the use of inherently quantum mechanical phenomena to perform information processing tasks that cannot be achieved using conventional classical information technologies. One famous example is quantum…

Quantum Physics · Physics 2007-05-23 J. A. Jones

We present a computer simulation study on the crystal nucleation process in suspensions of hard spheres, fully taking into account the solvent hydrodynamics. If the dynamics of collodial crystallization were purely diffusive, the crystal…

Soft Condensed Matter · Physics 2015-06-12 Marc Radu , Tanja Schilling

Nuclear-spin qubits have long coherence time and are desirably applied into quantum information processing. However, the existing methods either fail to address single nucleus (such as nuclear magnetic resonance), or severely affect nuclear…

Quantum Physics · Physics 2021-11-30 Jian Leng , Fan Yang , Xiang-Bin Wang

Solid-state spin qubits have emerged as promising platforms for quantum information. Despite extensive efforts in controlling noise in spin qubit quantum applications, one important but less controlled noise source is near-field…

Quantum Physics · Physics 2024-09-18 Wenbo Sun , Sathwik Bharadwaj , Runwei Zhou , Dan Jiao , Zubin Jacob

The nuclear spins in nanostructured semiconductors play a central role in quantum applications. The nuclear spins represent a useful resource for generating local magnetic fields but nuclear spin noise represents a major source of dephasing…

Nuclear magnetic resonance (NMR) has been widely used in the context of quantum information processing (QIP). However, despite the great similarities between NMR and nuclear quadrupole resonance (NQR), no experimental implementation for QIP…