Related papers: Single Molecule Magnetic Resonance and Quantum Com…
This chapter takes a microscopic view of quantum tunneling of magnetization (QTM) in single-molecule magnets (SMMs), focusing on the interplay between exchange and anisotropy. Careful consideration is given to the relationship between…
Magnetic resonance in an ensemble of laser-cooled trapped Rb atoms is excited using a micro- cantilever with a magnetic tip. The cantilever is mounted on a multi-layer chip designed to capture, cool, and magnetically transport cold atoms.…
We review the problem of spin decoherence of magnetic atoms deposited on a surface. Recent breakthroughs in scanning tunnelling microscopy (STM) make it possible to probe the spin dynamics of individual atoms, either isolated or integrated…
Atomic Parity Violation provides the rare opportunity of a low energy window into possible new fundamental processes at very high mass scales normally investigated at large high energy accelerators. Precise measurements on atomic systems…
Spin is commonly thought to reflect the true quantum nature of microphysics. We show that spin is related to intrinsic and field-like properties of single particles. These properties change continuously in external magnetic fields.…
We propose a scheme to engineer an effective spin Hamiltonian starting from a system of electrons confined in micro-Penning traps. By means of appropriate sequences of electromagnetic pulses, alternated to periods of free evolution, we…
Nonlinear manipulation of nuclear and electron spins is the basis for all advanced methods in magnetic resonance including multidimensional nuclear magnetic and electron spin resonance spectroscopies, magnetic resonance imaging, and in…
The simulation of the spectra measured in nuclear magnetic resonance (NMR) spectroscopy experiments is a computationally non-trivial problem which, due to its natural interpretation as a quantum spin problem, maps in a straightforward way…
Cold molecules provide an excellent platform for quantum information, cold chemistry, and precision measurement. Certain molecules have enhanced sensitivity to beyond Standard Model physics, such as the electron's electric dipole moment…
The loss of information about the relative phase between two quantum states, known as decoherence, strongly limits resolution in electron paramagnetic spectroscopy and hampers the use of molecules for quantum information processing. At low…
It is proposed to shoot a molecule through a pipe of mesoscopic scale. The molecule should effectifely carry two spins and antiferromagnetic chains should be embedded in the wall of the tube. If the momentum is detected before and behind…
Many things will have to go right for quantum computation to become a reality in the lab. For any of the presently-proposed approaches involving spin states in solids, an essential requirement is that these spins should be measured at the…
Single-molecule pulling techniques have emerged as versatile tools for probing the noncovalent forces holding together the secondary and tertiary structure of macromolecules. They also constitute a way to study at the single-molecule level…
Controlling quantum spins using electric rather than magnetic fields promises significant architectural advantages for developing quantum technologies. In this context, spins in molecular nanomagnets offer tunability of spin-electric…
Polar molecules are desirable systems for quantum simulations and cold chemistry. Molecular ions are easily trapped, but a bias electric field applied to polarize them tends to accelerate them out of the trap. We present a general solution…
Molecules are the most demanding quantum systems to be simulated by quantum computers because of their complexity and the emergent role of quantum nature. The recent theoretical proposal of Huh et al. (Nature Photon., 9, 615 (2015)) showed…
It is demonstrated that nuclear magnetic resonance experiments using pseudopure spin states can give possible outcomes of projective quantum measurement and probabilities of such outcomes. The physical system is a cluster of six…
The use of single molecules to design electronic devices is an extremely challenging and fundamentally different approach to further downsizing electronic circuits. Two-terminal molecular devices such as diodes were first predicted [1] and,…
A Mn4 single-molecule magnet (SMM) is used to show that quantum tunneling of magnetization (QTM) is not suppressed by moderate three dimensional exchange coupling between molecules. Instead, it leads to an exchange bias of the quantum…
A mechanism for creating well-collimated beams of neutral particles or atoms with spins is studied. The consideration is accomplished for a general realistic case, taking into account: (i) the finiteness of a cylindrical trap where the…