Related papers: Weisskopf-Wigner model for wave packet excitation
We present a mesoscopic model for reactive shock waves, which extends a previous model proposed in [G. Stoltz, Europhys. Lett. 76 (2006), 849]. A complex molecule (or a group of molecules) is replaced by a single mesoparticle, evolving…
We demonstrate experimentally the resonant excitation of plasma waves by trains of laser pulses. We also take an important first step to achieving an energy recovery plasma accelerator by showing that unused wakefield energy can be removed…
Motivated by ongoing pump-probe spectroscopy experiments, this work develops a theoretical framework for describing the rovibrational wave packet dynamics that ensues when a single weakly-bound van der Waals trimer is exposed to a short,…
We analyze the time-dependent interaction between a two-level atom and a spectrally encoded single-photon wave packet using the Heisenberg-Langevin equations and derive the atomic excitation probability. Spectral phase encoding broadens the…
An electron injector concept for laser-plasma accelerator was developed in ref [1] and [2] ; it relies on the use of counter-propagating ultrashort laser pulses. In [2], the scheme is as follows: the pump laser pulse generates a large…
This paper describes a method to do ab initio molecular dynamics in electronically excited systems within the random phase approximation (RPA). Using a dynamical variational treatment of the RPA frequency, which corresponds to the…
A three-dimensional, space-frequency model for the excitation of electromagnetic radiation in a free-electron laser is presented. The approach is applied in a numerical particle code WB3D, simulating the interaction of a free-electron laser…
In this work we review the Weisskopf-Wigner formalism for spontaneous emission considering the spatial modes of light as well as external atomic degrees of freedom which we introduce in the theory by modeling the atom as a wavepacket in…
We propose a methodology to design Wigner representations in phase spaces with nontrivial topology having evolution equations with desired mathematical properties. As an illustration, two representations of molecular rotations are developed…
We discuss a method to follow step-by-step time evolution of atomic and molecular systems based on QED (Quantum Electrodynamics). Our strategy includes expanding the electron field operator by localized wavepackets to define creation and…
This chapter gives an introduction to qualitative and quantitative topological analyses of molecular electronic transitions. Among the possibilities for qualitatively describing how the electronic structure of a molecule is reorganized upon…
We propose a simple way to determine the periodicities of wave packets in quantum systems directly from the energy differences of the states involved. The resulting classical periods and revival times are more accurate than those obtained…
The quantum state of a light beam can be represented as an infinite dimensional density matrix or equivalently as a density on the plane called the Wigner function. We describe quantum tomography as an inverse statistical problem in which…
We study the dynamics of a single excitation coherently shared amongst an ensemble of atoms and coupled to a one-dimensional wave guide. The coupling between the matter and the light field gives rise to collective phenomena such as…
This is the first in a series of two papers investigating the effect of electron-phonon coupling in two-dimensional Fourier transformed electronic spectroscopy. We present a series of one- and two-dimensional nonlinear spectroscopic…
The swing-up of quantum emitter population (SUPER) scheme allows to populate the excited state of a quantum emitter with near-unity fidelity using two red-detuned laser pulses. Its off-resonant, yet fully coherent nature has attracted…
The process of excitation of Cherenkov electromagnetic radiation by a laser pulse in ion dielectrics is investigated. Nonlinear electric polarization in isotropic ion dielectric medium and, accordingly, polarization charges and currents…
We report on generation of a rotational wavepacket in the ground vibronic state (v = 0) of excited electronic B2{\Sigma}u+ state of N2+ in a femtosecond laser induced plasma spark. Decoding of the rotational wavepacket is achieved with the…
The velocity of a passive particle in a one-dimensional wave field is shown to converge in law to a Wiener process, in the limit of a dense wave spectrum with independent complex amplitudes, where the random phases distribution is invariant…
The dynamics of excitonic energy transfer in molecular complexes triggered by interaction with laser pulses offers a unique window into the underlying physical processes. The absorbed energy moves through the network of interlinked pigments…