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Non-radiative energy transfer between a Rydberg atom and a polar molecule can be controlled by a DC electric field. Here we show how to exploit this control for state-resolved, non-destructive detection and spectroscopy of the molecules…

Atomic Physics · Physics 2023-11-28 Sabrina Patsch , Martin Zeppenfeld , Christiane P. Koch

Rydberg atoms have shown significant promise as the basis for highly sensitive detectors of continuous radio-frequency (RF) E-fields. Here, we study their time-dependent response to pulse-modulated RF E-fields at 19.4 GHz using a cesium…

Atomic Physics · Physics 2022-03-04 Stephanie M. Bohaichuk , Donald Booth , Kent Nickerson , Harry Tai , James P. Shaffer

This study explores the excitation and ionization of an atomic beam as a pathway to optimize focused ion beams (FIBs) for high-precision applications. Leveraging the unique advantages of Rydberg excitation followed by field ionization --…

Mean-field energy-level shifts arising as a result of strong electrostatic dipole interactions within dilute gases of polarized helium Rydberg atoms have been probed by microwave spectroscopy. The Rydberg states studied had principal…

Atomic Physics · Physics 2016-11-28 V. Zhelyazkova , R. Jirschik , S. D. Hogan

We present an experimental and theoretical study of the chaotic ionization of quasi-one-dimensional potassium Rydberg wavepackets via a phase-space turnstile mechanism. Turnstiles form a general transport mechanism for numerous chaotic…

Atomic Physics · Physics 2015-05-28 Korana Burke , Kevin A. Mitchell , Brendan Wyker , Shuzhen Ye , F. Barry Dunning

We theoretically investigate trapped ions interacting with atoms that are coupled to Rydberg states. The strong polarizabilities of the Rydberg levels increases the interaction strength between atoms and ions by many orders of magnitude, as…

Quantum Physics · Physics 2016-07-27 Thomas Secker , Rene Gerritsma , Alexander W. Glaetzle , Antonio Negretti

We propose and analyze a scheme for manipulating the propagation of single photon pulses with two polarization components in a Rydberg atomic gas via double electromagnetically induced transparency. We show that by storing a gate photon in…

Quantum Physics · Physics 2024-01-15 Ou Yao , Huang Guoxiang

It is clearly important to pursue atomic standards for quantities like electromagnetic fields, time, length and gravity. We have recently shown, using Rydberg states, that Rb atoms in a vapor cell can serve as a practical, compact standard…

Atomic Physics · Physics 2015-06-15 J. Sedlacek , A. Schwettmann , Harald Kübler , J. P. Shaffer

Rydberg atom-based radio frequency electromagnetic field sensors are drawing wide-spread interest because of their unique properties, such as small size, dielectric construction, and self-calibration. These photonic sensors use lasers to…

We introduce a scheme to entangle Rydberg ions in a linear ion crystal, using the high electric polarizability of the Rydberg electronic states in combination with mutual Coulomb coupling of ions that establishes common modes of motion.…

Atomic Physics · Physics 2019-10-16 Jonas Vogel , Weibin Li , Arezoo Mokhberi , Igor Lesanovsky , Ferdinand Schmidt-Kaler

We have studied the associative ionization of a Rydberg atom and a ground state atom in an ultracold Rydberg gas. The measured scattering cross section is three orders of magnitude larger than the geometrical size of the produced molecule.…

Atomic Physics · Physics 2017-08-24 Thomas Niederprüm , Oliver Thomas , Torsten Manthey , Tobias M. Weber , Herwig Ott

Selective field ionization is used to determine the state or distribution of states to which a Rydberg atom is excited. By evolving a small perturbation to the ramped electric field using a genetic algorithm, the shape of the time-resolved…

We present an entanglement scheme for Rydberg atoms using the van der Waals interaction phase induced by Ramsey-type pulsed interactions. This scheme realizes not only controlled phase operations between atoms at a distance larger than…

Atomic Physics · Physics 2020-01-29 Hanlae Jo , Yunheung Song , Minhyuk Kim , Jaewook Ahn

We describe a method for controlling many-body states in extended ensembles of Rydberg atoms, forming crystalline structures during laser excitation of a frozen atomic gas. Specifically, we predict the existence of an excitation number…

Atomic Physics · Physics 2015-05-14 T. Pohl , E. Demler , M. D. Lukin

Rydberg atoms in dc electric fields acquire static dipole moments. When the atoms are close to a surface producing an inhomogeneous electric field, such as by the adsorbates on an atom chip, depending on the sign of the dipole moment of the…

We investigate an ensemble of atoms which can be excited into a Rydberg state. Using a disordered quantum Ising model, we perform a numerical simulation of the experimental procedure and calculate the probability distribution function…

Quantum Gases · Physics 2012-10-08 David Breyel , Thomas L. Schmidt , Andreas Komnik

It is well-known from numerical and experimental results that the fraction of Rydberg states (excited neutral atoms) created by tunnel ionization declines dramatically with increasing ellipticity of laser light. We present a method to…

We propose a new technique to fully characterize the temporal structure of extreme ultraviolet pulses by ionizing a bound coherent electronic wavepacket. The populated energy levels make it possible to interfere different spectral…

Optics · Physics 2016-07-19 Stefan Pabst , Jan Marcus Dahlström

Rydberg atom-based electric field sensing can provide all-optical readout of radio frequency fields in a dielectric environment. However, because a single set of optical fields is typically used to prepare the Rydberg state and read out its…

Two-dimensional (2D) spectroscopy uses multiple electromagnetic pulses to infer the properties of a complex system. A paradigmatic class of target systems are molecular aggregates, for which one can obtain information on the eigenstates,…