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Magnetic noise of atomic nuclear spins is a major problem for solid state spin qubits. Highly-polarized nuclei would not only overcome this obstacle, but also make nuclear spins a useful quantum information resource. However, achieving…

Magnetic resonance imaging in ultra-low fields is often limited by mediocre signal-to-noise ratio hindering a higher resolution. Overhauser dynamic nuclear polarisation (O-DNP) using nitroxide radicals has been an efficient solution for…

We report on further investigation of nuclear hyperpolarization of helium-3 in magnetized plasma at a magnetic field of 3.66 T and at different experimental conditions in a dual cell of relatively large volume, compared to those reported in…

Atomic Physics · Physics 2022-08-16 Alexander Makarchenko , Vyacheslav Kuzmin , Kajum Safiullin , Murat Tagirov

The nature of the nano-scale environment presents a major challenge for solid-state implementation of spin-based qubits. In this work, a single electron spin in an optically pumped nanometer-sized III-V semiconductor quantum dot is used to…

Current-induced electron spin polarization is shown to produce nuclear hyperpolarization through dynamic nuclear polarization. Saturated fields of several millitesla are generated upon the application of electric field over a timescale of a…

Mesoscale and Nanoscale Physics · Physics 2014-10-31 C. J. Trowbridge , B. M. Norman , Y. K. Kato , D. D. Awschalom , V. Sih

Efficient polarization of organic molecules is of extraordinary relevance when performing nuclear magnetic resonance (NMR) and imaging. Commercially available routes to dynamical nuclear polarization (DNP) work at extremely…

Polarizing nuclear spins is of fundamental importance in biology, chemistry and physics. Methods for hyperpolarizing 13C nuclei from free electrons in bulk, usually demand operation at cryogenic temperatures. Room-temperature approaches…

Nuclear spins nearby nitrogen-vacancy (NV) centers in diamond are excellent quantum memory for quantum computing and quantum sensing, but are difficult to be initialized due to their weak interactions with the environment. Here we propose…

Quantum Physics · Physics 2019-09-04 Nanyang Xu , Yu Tian , Bing Chen , Jianpei Geng , Xiaoxiong He , Ya Wang , Jiangfeng Du

We polarize nuclear spins in a GaAs double quantum dot by controlling two-electron spin states near the anti-crossing of the singlet (S) and m_S=+1 triplet (T+) using pulsed gates. An initialized S state is cyclically brought into resonance…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. R. Petta , J. M. Taylor , A. C. Johnson , A. Yacoby , M. D. Lukin , C. M. Marcus , M. P. Hanson , A. C. Gossard

Dissolution Dynamic Nuclear Polarisation (dDNP) increases the sensitivity of magnetic resonance experiments by $>10^4$-fold, permitting isotopically-labelled molecules to be transiently visible in MRI scans. dDNP requires a source of…

We investigate the dynamic nuclear polarization process by frequently injecting polarized electron spins into a quantum dot. Due to the suppression of the direct dipolar and indirect electron-mediated nuclear spin interactions, by the…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Na Wu , Wenkui Ding , Anqi Shi , Wenxian Zhang

High-fidelity multi-qubit initialization is vital for quantum simulation, quantum information processing (QIP), and quantum sensing. In diamond platforms, nuclear spin registers can be initialized through polarization transfer from a nearby…

Quantum Physics · Physics 2026-03-02 Soham Pal , Oliver T. Whaites , Wolfgang Knolle , Tania S. Monteiro , Helena S. Knowles

The nuclear spin in the vicinity of a nitrogen-vacancy (NV) center possesses of long coherence time and convenient manipulation assisted by the strong hyperfine interaction with the NV center. It is suggested for the subsequent quantum…

Quantum Physics · Physics 2018-04-18 Yang-Yang Wang , Jing Qiu , Ying-Qi Chu , Mei Zhang , Jianming Cai , Qing Ai , Fu-Guo Deng

We determine the polarization of the bulk $^{13}$C nuclear spin system in diamond produced by interaction with optically oriented nitrogen-vacancy (NV-) defect centers. $^{13}$C nuclei are polarized into the higher energy Zeeman state with…

Other Condensed Matter · Physics 2015-05-14 Jonathan P. King , Patrick J. Coles , Jeffrey A. Reimer

We investigate dynamic nuclear polarization in quantum point contacts (QPCs) in the integer and fractional quantum Hall regimes. Following the application of a dc bias, fractional plateaus in the QPC shift symmetrically about half filling…

Mesoscale and Nanoscale Physics · Physics 2014-11-20 A. Kou , D. T. McClure , C. M. Marcus , L. N. Pfeiffer , K. W. West

We demonstrate dynamical nuclear spin polarization in the absence of an external magnetic field, by resonant circularly polarized optical excitation of a single electron or hole charged quantum dot. Optical pumping of the electron spin…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 C. W. Lai , P. Maletinsky , A. Badolato , A. Imamoglu

It is demonstrated that the time evolution of the electron-nuclear polarization transfer process during pulsed dynamic nuclear polarization (DNP) can be reversed on a microsecond timescale, leading to the observation of DNP echoes. The DNP…

Chemical Physics · Physics 2024-06-28 Nino Wili , Anders B. Nielsen , José P. Carvalho , Niels Chr. Nielsen

Dynamic nuclear polarization (DNP) of molecules in a solution at room temperature has potential to revolutionize nuclear magnetic resonance spectroscopy and imaging. The prevalent methods for achieving DNP in solutions are typically most…

Chemical Physics · Physics 2016-03-02 Qiong Chen , Ilai Schwarz , Fedor Jelezko , Alex Retzker , Martin B Plenio

Self-compensated comagnetometers, employing overlapping samples of spin-polarized alkali and noble gases (for example K-$^3$He) are promising sensors for exotic beyond-the-standard-model fields and high-precision metrology such as rotation…

Rapid injection of spin polarization into an ensemble of nuclear spins is a problem of broad interest, spanning dynamic nuclear polarization (DNP) to quantum information science. We report on a strategy to boost the spin injection rate by…