Related papers: Precise Control of Molecular Dynamics with a Femto…
We demonstrate the use of a femtosecond frequency comb to coherently drive stimulated Raman transitions between terahertz-spaced atomic energy levels. More specifically, we address the $3d~^2D_{3/2}$ and $3d~^2D_{5/2}$ fine structure levels…
We report on coherent control of excitation processes of translationally ultracold rubidium dimers in a magneto-optical trap by using shaped femtosecond laser pulses. Evolution strategies are applied in a feedback loop in order to optimize…
Quantum coherent control (1-3) is a powerful tool for steering the outcome of quantum processes towards a desired final state, by accurate manipulation of quantum interference between multiple pathways. Although coherent control techniques…
We present an experiment demonstrating high-resolution coherent control of a four-level atomic system in a closed (diamond) type configuration. A femtosecond frequency comb is used to establish phase coherence between a pair of two-photon…
Coherent control of the atomic two-photon absorption with shaped single-cycle pulses is examined theoretically in the weak-field regime. The control over the stabilized carrier-envelope phase (CEP) of the pulses is determined as a key…
Optical frequency combs are laser sources which are capable of generating discrete, equal-spaced and highly coherent comb modes. Optical frequency comb technique provides a significant bridge to transfer the stability between optical…
We demonstrate high resolution coherent control of cold atomic Rubidium utilizing spectral phase manipulation of a femtosecond optical frequency comb. Transient coherent accumulation is directly manifested by the enhancement of signal…
Coherent control of femtosecond two-photon absorption in the intermediate-field regime is analyzed in detail in the powerful frequency domain using an extended 4th-order perturbative description. The corresponding absorption is coherently…
We show that a single femtosecond optical frequency comb may be used to induce two-photon transitions between molecular vibrational levels to form ultracold molecules, e.g., KRb. The phase across an individual pulse in the pulse train is…
Quantum coherent control of ultrafast bond making and the subsequent molecular dynamics is crucial for the realization of a new photochemistry, where a shaped laser field is actively driving the chemical system in a coherent way from the…
Coherent control of ultrafast molecule making from colliding reactants is crucial for realizing coherent control of binary photoreactions (CCBP). To handle diverse excitation scenarios, feasibility with both weak and strong fields is…
The classic self-referenced frequency comb acts as an unrivaled ruler for precision optical metrology in both time and frequency. Two decades after its invention, the frequency comb is now used in numerous active sensing applications. Many…
In recent experiments on ultracold matter, molecules have been produced from ultracold atoms by photoassociation, Feshbach resonances, and three-body recombination. The created molecules are translationally cold, but vibrationally highly…
We demonstrate the use of an optical frequency comb to coherently control and entangle atomic qubits. A train of off-resonant ultrafast laser pulses is used to efficiently and coherently transfer population between electronic and…
An efficient method to coherently control the waveforms of gamma-photons has been proposed and experimentally realized. It is based on the resonant interaction of gamma-photons with an ensemble of nuclei with modulated frequency of the…
Coherent control of two-state systems is traditionally achieved by resonant pulses of specific Rabi frequency and duration, by adiabatic techniques using level crossings or delayed pulses, or by sequences of pulses with precise relative…
Two techniques that employ equally spaced trains of optical pulses to map an optical high frequency into a low frequency modulation of the signal that can be detected in real time are compared. The development of phase-stable optical…
We have studied the effects of chirped femtosecond laser pulses on the formation of ultracold molecules in a Rb magneto-optical trap. We have found that application of chirped femtosecond pulses suppressed the formation of 85Rb-2 and 87Rb-2…
Along with the scaling of dimensions in quantum systems, transitions between the system's energy levels would become close in frequency, which are conventionally resolved by weak and lengthy pulses. Here, we extend and experimentally…
We describe a method for improving coherent control through the use of detailed knowledge of the system's Hamiltonian. Precise unitary transformations were obtained by strongly modulating the system's dynamics to average out unwanted…