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We observe the low-lying excitations of a molecular dimer formed by two electrons in a GaAs semiconductor quantum dot in which the number of confined electrons is tuned by optical illumination. By employing inelastic light scattering we…

Mesoscale and Nanoscale Physics · Physics 2010-06-16 Achintya Singha , Vittorio Pellegrini , Aron Pinczuk , Loren N. Pfeiffer , Ken W. West , Massimo Rontani

The biexciton cascade in a quantum dot can be used to generate entangled-photon pairs rapidly and deterministically (on demand). However, due to a large fine-structure splitting between intermediate exciton energy levels, which-path…

Mesoscale and Nanoscale Physics · Physics 2009-12-08 W. A. Coish , J. M. Gambetta

In a charge tunable device, we investigate the fine structure splitting of neutral excitons in single long-wavelength (1.1\mu m < \lambda < 1.3 \mu m) InGaAs quantum dots as a function of external uniaxial strain. Nominal fine structure…

To generate entangled photon pairs via quantum dots (QDs), the exciton fine structure splitting (FSS) must be comparable to the exciton homogeneous line width. Yet in the (In,Ga)As/GaAs QD, the intrinsic FSS is about a few tens $\mu$eV. To…

Materials Science · Physics 2009-11-13 Lixin He , Ming Gong , Chuan-Feng Li , Guang-Can Guo , Alex Zunger

We present an optical study of closely-spaced self-assembled InAs/GaAs quantum dots. The energy spectrum and correlations between photons subsequently emitted from a single pair provide not only clear evidence of coupling between the…

We show that with a new family of pyramidal site-controlled InGaAsN quantum dots it is possible to obtain areas containing as much as 15% of polarization-entangled photon emitters - a major improvement if compared to the small fraction…

Mesoscale and Nanoscale Physics · Physics 2014-02-10 Gediminas Juska , Valeria Dimastrodonato , Lorenzo O. Mereni , Agnieszka Gocalinska , Emanuele Pelucchi

Exciton fine-structure splittings within quantum dots introduce phase differences between the two biexciton decay paths that greatly reduce the entanglement of photon pairs generated via biexciton recombination. We analyze this problem in…

Quantum Physics · Physics 2015-03-13 Zong-Quan Zhou , Chuan-Feng Li , Geng Chen , Jian-Shun Tang , Yang Zou , Ming Gong , Guang-Can Guo

The multi-excitonic decay process in a single InAs quantum dot is studied through high-resolution time-resolved spectroscopy. A cascaded emission sequence involving three spectral lines is seen that is described well over a wide range of…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Charles Santori , Glenn S. Solomon , Matthew Pelton , Yoshihisa Yamamoto

Entangled photon pairs are key to many novel applications in quantum technologies. Semiconductor quantum dots can be used as sources of on-demand, highly entangled photons. The fidelity to a fixed maximally entangled state is limited by the…

We discuss the influence of a rapid thermal annealing step on the magneto-optical emission properties of In(Ga)As/GaAs quantum dots. We map out a strong influence of the growth- and anneling parameters on the quantum excitons' effective…

Mesoscale and Nanoscale Physics · Physics 2016-05-25 T. Braun , S. Betzold , N. Lundt , M. Kamp , S. Höfling , C. Schneider

The entanglement between photon pairs generated from the biexciton cascade transition in a semi- conductor quantum dot located in the vicinity of a metal nanoparticle is theoretically investigated. In the model scheme, the biexciton-exciton…

Quantum Physics · Physics 2017-09-20 Tara Moradi , Malek Bagheri Harouni , Mohammad Hossein Naderi

The temperature-dependent electron spin relaxation of positively charged excitons in a single InAs quantum dot (QD) was measured by time-resolved photoluminescence spectroscopy at zero applied magnetic fields. The experimental results show…

Mesoscale and Nanoscale Physics · Physics 2015-06-03 X. M. Dou , B. Q. Sun , D. S. Jiang , H. Q. Ni , Z. C. Niu

Single and multi-band (Burt-Foreman) k.p Hamiltonians for GaAs crystal phase quantum dots are developed and used to assess ongoing experimental activity on the role of such factors as quantum confinement, spontaneous polarization, valence…

Mesoscale and Nanoscale Physics · Physics 2016-04-04 Juan I. Climente , Carlos Segarra , Fernando Rajadell , Josep Planelles

In this paper, we study the exciton absorption spectra in InGaAs prolate ellipsoidal quantum dots when a strong pump laser resonant with electron quantized levels is active. Our obtained results by renormalized wavefunction theory show…

Mesoscale and Nanoscale Physics · Physics 2021-03-02 Le Thi Ngoc Bao , Duong Dinh Phuoc , Le Thi Dieu Hien , Dinh Nhu Thao

A transition between the strong (coherent) and weak (incoherent) coupling limits of resonant interaction between quantum well (QW) excitons and bulk photons is analyzed and quantified as a function of the incoherent damping rate caused by…

Mesoscale and Nanoscale Physics · Physics 2008-03-04 C. Creatore , A. L. Ivanov

We theoretically investigate the joint photodetection probabilities of the biexciton-exciton cascade in single semiconductor quantum dots and analytically derive the density matrix and the Bell's inequalities of the entangled state. Our…

Optics · Physics 2009-11-13 Matthieu Larqué , Isabelle Robert-Philip , Alexios Beveratos

We theoretically investigate the efficiency of an entanglement swapping procedure based on the use of quantum dots as sources of entangled photon pairs. The four-photon interference that affects such efficiency is potentially limited by the…

Mesoscale and Nanoscale Physics · Physics 2015-03-27 F. Troiani

We have studied theoretically the type-II GaAsSb capped InAs quantum dots for two structures differing in the composition of the capping layer, being either (i) constant or (ii) with Sb accumulation above the apex of the dot. We have found…

Mesoscale and Nanoscale Physics · Physics 2023-07-19 P. Klenovsky , V. Krapek , J. Humlicek

Semiconductor quantum dots are promising building blocks for quantum communication applications. Although deterministic, efficient, and coherent emission of entangled photons has been realized, implementing a practical quantum repeater…

Singlet fission, a process that splits a singlet exciton into a biexciton, has promise in quantum information. We report time-resolved electron paramagnetic resonance measurements on a molecule, TIPS-BP1$'$, designed to exhibit strongly…

Chemical Physics · Physics 2022-02-22 Ryan D. Dill , Kori E. Smyser , Niels H. Damrauer , Joel D. Eaves
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