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We introduce machine learning models of quantum mechanical observables of atoms in molecules. Instant out-of-sample predictions for proton and carbon nuclear chemical shifts, atomic core level excitations, and forces on atoms reach…

Chemical Physics · Physics 2015-08-26 Matthias Rupp , Raghunathan Ramakrishnan , O. Anatole von Lilienfeld

Many standard linear algebra problems can be solved on a quantum computer by using recently developed quantum linear algebra algorithms that make use of block encodings and quantum eigenvalue/singular value transformations. A block encoding…

Quantum Physics · Physics 2023-05-23 Daan Camps , Lin Lin , Roel Van Beeumen , Chao Yang

The basic idea of quantum computing is surprisingly similar to that of kernel methods in machine learning, namely to efficiently perform computations in an intractably large Hilbert space. In this paper we explore some theoretical…

Quantum Physics · Physics 2019-02-06 Maria Schuld , Nathan Killoran

From the existence of an efficient quantum algorithm for factoring, it is likely that quantum computation is intrinsically more powerful than classical computation. At present, the best upper bound known for the power of quantum computation…

Quantum Physics · Physics 2015-09-14 Ciarán M. Lee , Jonathan Barrett

Quantum computing is concerned with computer technology based on the principles of quantum mechanics, with operations performed at the quantum level. Quantum computational models make it possible to analyze the resources required for…

Formal Languages and Automata Theory · Computer Science 2019-01-24 Amandeep Singh Bhatia , Ajay Kumar

First principles based exploration of chemical space deepens our understanding of chemistry, and might help with the design of new materials or experiments. Due to the computational cost of quantum chemistry methods and the immens number of…

Chemical Physics · Physics 2020-08-18 Bing Huang , O. Anatole von Lilienfeld

A typical oracle problem is finding which software program is installed on a computer, by running the computer and testing its input-output behaviour. The program is randomly chosen from a set of programs known to the problem solver. As…

Quantum Physics · Physics 2007-05-23 Giuseppe Castagnoli

Quantum computers hold promise to enable efficient simulations of the properties of molecules and materials; however, at present they only permit ab initio calculations of a few atoms, due to a limited number of qubits. In order to harness…

Materials Science · Physics 2020-07-07 He Ma , Marco Govoni , Giulia Galli

Many quantum algorithms for numerical linear algebra assume black-box access to a block-encoding of the matrix of interest, which is a strong assumption when the matrix is not sparse. Kernel matrices, which arise from discretizing a kernel…

Quantum Physics · Physics 2022-12-14 Quynh T. Nguyen , Bobak T. Kiani , Seth Lloyd

Quantum computers can execute algorithms that dramatically outperform classical computation. As the best-known example, Shor discovered an efficient quantum algorithm for factoring integers, whereas factoring appears to be difficult for…

Quantum Physics · Physics 2010-01-19 Andrew M. Childs , Wim van Dam

A central task in the field of quantum computing is to find applications where quantum computer could provide exponential speedup over any classical computer. Machine learning represents an important field with broad applications where…

Quantum Physics · Physics 2017-11-07 Xun Gao , Zhengyu Zhang , Luming Duan

Recently developed quantum algorithms suggest that quantum computers can solve certain problems and perform certain tasks more efficiently than conventional computers. Among other reasons, this is due to the possibility of creating…

Quantum Physics · Physics 2007-05-23 Rolando D. Somma

Quantum algorithm involves the manipulation of amplitudes and computational basis, of which manipulating basis is largely a quantum analogue of classical computing that is always a major contributor to the complexity. In order to make full…

In quantum chemistry, the price paid by all known efficient model chemistries is either the truncation of the Hilbert space or uncontrolled approximations. Theoretical computer science suggests that these restrictions are not mere…

Chemical Physics · Physics 2017-03-15 James D. Whitfield , Peter J. Love , Alan Aspuru-Guzik

Group convolutions and cross-correlations, which are equivariant to the actions of group elements, are commonly used in mathematics to analyze or take advantage of symmetries inherent in a given problem setting. Here, we provide efficient…

We develop a formal model for distributed measurement-based quantum computations, adopting an agent-based view, such that computations are described locally where possible. Because the network quantum state is in general entangled, we need…

Quantum Physics · Physics 2007-05-23 Vincent Danos , Ellie D'Hondt , Elham Kashefi , Prakash Panangaden

The natural Hilbert Space of quantum particles can implement maximum-likelihood (ML) decoding of classical information. The 'Quantum Product Algorithm' (QPA) is computed on a Factor Graph, where function nodes are unitary matrix operations…

Quantum Physics · Physics 2007-05-23 Matthew G. Parker

Chemistry and materials science are widely regarded as potential killer application fields for quantum hardware. While the dream of unlocking unprecedented simulation capabilities remains compelling, quantum algorithm development must adapt…

Quantum Physics · Physics 2026-03-20 Davide Castaldo , Markus Reiher

A dynamical quantum model assigns an eigenstate to a specified observable even when no measurement is made, and gives a stochastic evolution rule for that eigenstate. Such a model yields a distribution over classical histories of a quantum…

Quantum Physics · Physics 2007-05-23 Scott Aaronson

Error correction will add so much overhead to large quantum computations that we suspect the most efficient algorithms will use a classical co-processor to do as much work as possible. We present a method to offload portions of a quantum…

Quantum Physics · Physics 2020-08-12 Samuel Jaques , Craig Gidney