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Related papers: Electronic energy transfer: vibrational control an…

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Organic molecules store the energy of absorbed light in the form of charge-neutral molecular excitations -- Frenkel excitons. Usually, in amorphous organic materials, excitons are viewed as quasiparticles, localized on single molecules,…

Mesoscale and Nanoscale Physics · Physics 2013-04-02 Semion K. Saikin , Alexander Eisfeld , Stéphanie Valleau , Alán Aspuru-Guzik

A general rate theory for resonance energy transfer is formulated to incorporate any degrees of freedom (e.g., rotation, vibration, exciton, and polariton) as well as coherently-coupled composite states. The compact rate expression allows…

Chemical Physics · Physics 2022-01-31 Jianshu Cao

We investigate the time evolution of statistical properties of a single mode radiation field after its interaction with a two-level atom. The entire system is described by a dispersive Jaynes-Cummings Hamiltonian assuming the atomic state…

Quantum Physics · Physics 2020-12-07 C. J. S. Ferreira , C. Valverde , B. Baseia

Turbulent dissipation is considered a main source of heating and acceleration in cosmological plasmas. The alternating current Joule-like term, $\langle\delta j \cdot \delta E\rangle$, is used to measure the energy transfer between…

Space Physics · Physics 2021-03-17 Die Duan , Jiansen He , Honghong wu , Daniel Verscharen

We study the motion (translational, vibrational, and rotational) of a diatomic impurity immersed in an electron liquid and exposed to electronic current. An approach based on the linear response time-dependent density functional theory…

Materials Science · Physics 2024-07-12 Vladimir U. Nazarov , Tchavdar N. Todorov , E. K. U. Gross

The coupling of the charge carriers passing through a molecule bridging two bulky conductors with local vibrational modes of the molecule, gives rise to distinct features in the electronic transport properties on one hand, and to…

Mesoscale and Nanoscale Physics · Physics 2017-02-01 A. Ueda , Y. Utsumi , Y. Tokura , O. Entin-Wohlman , A. Aharony

The empirical valence bond (EVB) method [J. Chem. Phys. 52, 1262 (1970)] has always embodied charge transfer processes. The mechanism of that behavior is examined here and recast for use as a new empirical potential energy surface for…

Chemical Physics · Physics 2009-11-10 Steven M. Valone , Susan R. Atlas

Simulation of a system consisted of free particle bouncing on a vertically vibrated based is performed. Two different states, which are steady and unsteady energy transfer state are found. The vibrating based is hold at constant vibration…

Soft Condensed Matter · Physics 2011-06-10 Suparno Satira , Sparisoma Viridi , Freddy P Zen

We demonstrate that charge separation at donor-acceptor interfaces is a complex process that is controlled by the combined action of Coulomb binding for electron-hole pairs and partial relaxation due to quantized phonons. A joint…

Materials Science · Physics 2015-09-07 Soumya Bera , Nicolas Gheeraert , Simone Fratini , Sergio Ciuchi , Serge Florens

The influence of an electron-vibrational coupling on the laser control of electron transport through a molecular wire that is attached to several electronic leads is investigated. These molecular vibrational modes induce an effective…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Jörg Lehmann , Sigmund Kohler , Volkhard May , Peter Hänggi

We present a real-time path integral theory for the rate of electron transfer reactions. Using graph theoretic techniques, the dynamics is expressed in a formally exact way as a set of integral equations. With a simple approximation for the…

chem-ph · Physics 2009-10-28 Juergen T. Stockburger , C. H. Mak

We study the interplay between two environmental influences on excited state energy transfer in photosynthetic light harvesting complexes, namely, vibrationally assisted energy transfer (VAET) and environment-assisted quantum transport…

Biological Physics · Physics 2022-03-28 Zeng-Zhao Li , Liwen Ko , Zhibo Yang , Mohan Sarovar , K. Birgitta Whaley

We study charge and energy transfer in two-site molecular electronic junctions in which electron transport is assisted by a vibrational mode. To understand the role of mode harmonicity/anharmonicity on transport behavior, we consider two…

Mesoscale and Nanoscale Physics · Physics 2015-09-01 Bijay Kumar Agarwalla , Jian-Hua Jiang , Dvira Segal

We experimentally study the vicinity of the Jamming transition by investigating the statics and the dynamics of the contact network of an horizontally shaken bi-disperse packing of photo-elastic discs. Compressing the packing very slowly,…

Soft Condensed Matter · Physics 2015-06-04 C. Coulais , R. P. Behringer , O. Dauchot

Electronic excitation energy transfer along a molecular wire depends on the relative orientation of the electronic transition dipole moments of neighboring chromophores. In porphycenes this orientation is changed upon double proton transfer…

Chemical Physics · Physics 2010-10-28 Mahmoud K. Abdel-Latif , Oliver Kuehn

Recent ultrafast optical experiments show that excitons in large biological light-harvesting complexes are coupled to molecular vibration modes. These high-frequency vibrations will not only affect the optical response, but also drive the…

Quantum Physics · Physics 2015-02-12 Arend G. Dijkstra , Chen Wang , Jianshu Cao , Graham R. Fleming

Using molecular simulation and continuum dielectric theory, we consider how electrochemical kinetics are modulated by twist angle in bilayer graphene electrodes. By establishing a connection between twist angle and the screening length of…

Statistical Mechanics · Physics 2024-11-06 Leonardo Coello Escalante , David T. Limmer

Strong light-matter coupling within an optical cavity leverages the collective interactions of molecules and confined electromagnetic fields, giving rise to the possibilities of modifying chemical reactivity and molecular properties. While…

Chemical Physics · Physics 2025-05-29 Shravan Kumar Sharma , Hsing-Ta Chen

We theoretically study pump-photon-energy-dependent pathways of a photoinduced dimer-Mott-insulator-to-metal transition, on the basis of numerical solutions to the time-dependent Schr\"odinger equation for the exact many-body wave function…

Strongly Correlated Electrons · Physics 2015-05-28 Kenji Yonemitsu , Satoshi Miyashita , Nobuya Maeshima

Real-time time-dependent density functional theory, in conjunction with the Ehrenfest molecular dynamics scheme, is becoming a popular methodology to investigate ultrafast phenomena on the nanoscale. Thanks to recent developments, it is…

Materials Science · Physics 2020-08-18 Jannis Krumland , Ana M. Valencia , Stefano Pittalis , Carlo A. Rozzi , Caterina Cocchi
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