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We study the F\"orster resonant energy transfer (FRET) rate in multichromophoric systems. The multichromophoric FRET rate is determined by the overlap integral of the donor's emission and acceptor's absorption spectra, which are obtained…

Biological Physics · Physics 2015-06-19 Jian Ma , Jianshu Cao

We explore the mechanism for the long-lived quantum coherence by considering the discrete phonon modes: these vibrational modes effectively weaken the exciton-environment interaction, due to the new composite (polaron) formed by excitons…

Chemical Physics · Physics 2017-07-10 Zhedong Zhang , Jin Wang

The dynamics of excitonic energy transfer in molecular complexes triggered by interaction with laser pulses offers a unique window into the underlying physical processes. The absorbed energy moves through the network of interlinked pigments…

Quantum Physics · Physics 2025-12-30 Tobias Kramer

The strong light-matter coupling of a microcavity mode to tightly bound Frenkel excitons in organic materials emerged as a versatile, room-temperature compatible platform to study nonlinear many-particle physics and bosonic condensation.…

The role of quantum coherence and the environment in the dynamics of excitation energy transfer is not fully understood. In this work, we introduce the concept of dynamical contributions of various physical processes to the energy transfer…

Quantum Physics · Physics 2009-07-18 Patrick Rebentrost , Masoud Mohseni , Alán Aspuru-Guzik

The decoherence induced on a single qubit by its interaction with the environment is studied. The environment is modelled as a scalar two-level boson system that can go through either first order or continuous excited state quantum phase…

Quantum Physics · Physics 2015-05-14 P. Perez-Fernandez , A. Relano , J. M. Arias , J. Dukelsky , J. E. Garcia-Ramos

Photons and electrons are the key quantum media for the quantum information processing based on solid state devices. The essential ingredients to accomplish the quantum repeater were investigated and their underlying physics were revealed.…

Mesoscale and Nanoscale Physics · Physics 2008-01-15 Toshihide Takagahara , Ozgur Cakir

We study nonadiabatic electron transfer within the biased spin-boson model. We calculate the incoherent transfer rate in analytic form at all temperatures for a power law form of the spectral density of the solvent coupling. In the Ohmic…

Statistical Mechanics · Physics 2009-10-31 G. Lang , E. Paladino , U. Weiss

We present numerically exact results for the quantum coherent energy transfer in the Fenna-Matthews-Olson molecular aggregate under realistic physiological conditions, including vibrational fluctuations of the protein and the pigments for…

Mesoscale and Nanoscale Physics · Physics 2011-12-06 Peter Nalbach , Daniel Braun , Michael Thorwart

F\"orster resonance energy transfer has an important role in nature and technology, rendering its exact theoretical understanding significant. To this end, a system of two electronically decoupled quantum dots (QDs) is considered,…

Mesoscale and Nanoscale Physics · Physics 2025-09-22 Liubov S. Sirkina , Luke M. J. Hall , Amy Morreau , Wolfgang Langbein , Egor A. Muljarov

With extensive variational simulations, dissipative quantum phase transitions in the sub-Ohmic spin-boson model are numerically studied in a dense limit of environmental modes. By employing a generalized trial wave function composed of…

Statistical Mechanics · Physics 2023-09-06 Yulong Shen , Nengji Zhou

We propose a physical principle for implementation of controllable interactions of identical electromagnetic bosons (excitons or polaritons) in two-dimensional (2D) semiconductors. The key ingredients are tightly bound biexcitons and…

Quantum Gases · Physics 2024-05-22 Sergueï V. Andreev

A 1-dimensional model for coherent quantum energy transfer through a complex of compressible boxes is investigated by numerical integration of the time-dependent Schr\"odinger equation. Energy is communicated from one box to the next by the…

Chemical Physics · Physics 2015-05-12 Mark A. Peterson

We report high time-resolution measurements of photon statistics from pairs of dye molecules coupled by fluorescence resonance energy transfer (FRET). In addition to quantum-optical photon antibunching, we observe photon bunching on a…

Condensed Matter · Physics 2009-11-07 Andrew J. Berglund , Andrew C. Doherty , Hideo Mabuchi

We show that the precise preparation of a quantum superposition between three rotational states of an ultracold dipolar molecule generates controllable interferences in their two-body scattering dynamics and collisional rate coefficients,…

Quantum Gases · Physics 2024-06-21 Thibault Delarue , Goulven Quéméner

We investigate the microscopic mechanism of quantum energy transfer in the nonequilibrium spin-boson model. By developing a nonequilibrium polaron-transformed Redfield equation based on fluctuation decoupling, we dissect the energy transfer…

Mesoscale and Nanoscale Physics · Physics 2015-08-11 Chen Wang , Jie Ren , Jianshu Cao

Based on concepts from quantum thermodynamics the two-level system coupled to a single electromagnetic mode is analyzed. Focusing on the case of detuning, where the mode frequency does not match the transition frequency, effective energies…

Quantum Physics · Physics 2022-02-02 Andreas Wacker

In organic semiconductors working under ambient circumstance, there are remarkable quantum effects lack of comprehensive understanding, and an exotic composite particle named charge transfer (CT) exciton is normally regarded as the key…

Mesoscale and Nanoscale Physics · Physics 2021-12-07 Yao Yao

Central spin models, where a single spinful particle interacts with a spin environment, find wide application in quantum information technology and can be used to describe, e.g., the decoherence of a qubit over time. We propose a method of…

Quantum Physics · Physics 2023-11-30 Jacek Dobrzyniecki , Michał Tomza

Quantum information processing has greatly increased interest in the phenomenon of environmentally-induced decoherence. The spin boson model is widely used to study the interaction between a spin-modelling a quantum particle moving in a…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Nicholas Wynn Watkins , David Waxman