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We demonstrate a wide-band all-optical method of nanoscale magnetic resonance (MR) spectroscopy under ambient conditions. Our method relies on cross-relaxation between a probe spin, the electronic spin of a nitrogen-vacancy centre in…

Numerically optimised microwave pulses are used to increase excitation efficiency and modulation depth in electron spin resonance experiments performed on a spectrometer equipped with an arbitrary waveform generator. The optimisation…

Chemical Physics · Physics 2018-10-19 David L. Goodwin , William K. Myers , Christiane R. Timmel , Ilya Kuprov

Ion adsorption and dynamics in porous carbons is crucial for many technologies such as energy storage and desalination. Nuclear Magnetic Resonance (NMR) spectroscopy is a key method to investigate such systems thanks to the possibility to…

Materials Science · Physics 2024-04-29 El Hassane Lahrar , Céline Merlet

We discuss the commonly encountered problem when optimizing NMR pulses using optimal control that the otherwise very precise NMR theory does not provide as excellent agreement with experiments. We hypothesize that this disagreement is due…

Dynamic nuclear polarization is widely used to enhance the sensitivity of nuclear magnetic resonance. It is presently the method of choice for enhancing the sensitivity of high-field solid state NMR experiments performed under cryogenic…

Chemical Physics · Physics 2022-02-02 Maria Grazia Concilio , Ilya Kuprov , Lucio Frydman

The polarisation dynamics of nuclear spins weakly coupled to an NV center is highly sensitive to the parameters of the microwave control and the nuclear Larmor frequency. What is commonly regarded as a challenge, we propose here as a…

Quantum Physics · Physics 2018-10-24 Q. Chen , Z. -Y. Wang , B. Tratzmiller , I. Schwartz , M. B. Plenio

NV-diamonds have attracted keen interest for nanoscale sensing and spin manipulation. In particular, the non-equilibrium electron spin polarization after optical excitation of single NV centers has successfully been transferred to nuclear…

Mesoscale and Nanoscale Physics · Physics 2021-11-24 R. Rizzato , F. Bruckmaier , K. S. Liu , S. J. Glaser , D. B. Bucher

Correlation functions are a standard tool for analyzing statistical particle trajectories. Recently, a so called mean back relaxation (MBR) has been introduced, which correlates positions at three time points. The deviation of its long time…

Statistical Mechanics · Physics 2024-10-07 Gabriel Knotz , Matthias Krüger

Nuclear magnetic resonance spectroscopy with solid-state spin sensors is a promising pathway for the detection of nuclear spins at the micro- and nanoscale. Although many nanoscale experiments rely on a single sensor spin for the detection…

We consider the optimal quantization of compressive sensing measurements following the work on generalization of relaxed belief propagation (BP) for arbitrary measurement channels. Relaxed BP is an iterative reconstruction scheme inspired…

Information Theory · Computer Science 2016-11-15 Ulugbek Kamilov , Vivek K Goyal , Sundeep Rangan

A model of dynamic orientation using optimized radiofrequency (RF) irradiation produced perpendicular to the holding field is developed for the spin-1 system required for tensor-polarized fixed-target experiments. The derivation applies to…

Nuclear Theory · Physics 2017-07-25 Dustin Keller

We demonstrate theoretically and numerically how to control the NMR relaxation rate after application of the standard spin echo technique. Using radiation damping, we return the nuclear magnetization to its equilibrium state during a time…

Instrumentation and Detectors · Physics 2011-12-01 Gennady P. Berman , Michelle A. Espy , Vyacheslav N. Gorshkov , Vladimir I. Tsifrinovich , Petr L. Volegov

The NMR relaxation rate $1/T_{1}$ is studied for one-dimensional multicomponent spin-orbital systems. By combining the bosonization techniques and the exact solution of the SU($n$) model, we evaluate the power-law exponent and the…

Strongly Correlated Electrons · Physics 2015-06-24 Akira Kawaguchi , Tatsuya Fujii , Norio Kawakami

Magnetosensitive spin-correlated radical-pairs (SCRPs) offer a promising platform for noise-robust quantum metrology. However, unavoidable interradical interactions, such as electron-electron dipolar and exchange couplings, alongside…

Quantum Physics · Physics 2026-02-25 Luke D. Smith , Farhan T. Chowdhury , Jonas Glatthard , Daniel R. Kattnig

Ensembles of nitrogen-vacancy (NV) centers are used as sensors to detect NMR signals from micron-sized samples at room temperature. In this scenario, the regime of large magnetic fields is especially interesting as it leads to a large…

Quantum Physics · Physics 2023-04-04 C. Munuera-Javaloy , A. Tobalina , J. Casanova

We study multiple-spin coherence transfers in linear Ising spin chains with nearest neighbor couplings. These constitute a model for efficient information transfers in future quantum computing devices and for many multi-dimensional…

Magnetic resonance (MR) fingerprinting is a new quantitative imaging paradigm, which simultaneously acquires multiple MR tissue parameter maps in a single experiment. In this paper, we present an estimation-theoretic framework to perform…

Signal Processing · Electrical Eng. & Systems 2018-10-03 Bo Zhao , Justin P. Haldar , Congyu Liao , Dan Ma , Yun Jiang , Mark A. Griswold , Kawin Setsompop , Lawrence L. Wald

Pulsed Dynamic Nuclear Polarization (DNP) is currently receiving substantial interest as a means to enhance the sensitivity of nuclear magnetic resonance (NMR) and magnetic resonance imaging (MRI) by orders of magnitude. It has also…

Spin noise sets fundamental limits to the precision of measurements using spin-polarized atomic vapors, such as performed with sensitive atomic magnetometers. Spin squeezing offers the possibility to extend the measurement precision beyond…

Atomic Physics · Physics 2009-11-13 I. K. Kominis

[1-13C]pyruvate is the most widely used tracer for hyperpolarized metabolic magnetic resonance imaging, with profound applications in tumor and inflammation diagnosis as well as treatment monitoring. The most fundamental hurdle to broader…