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The interaction of a weakly bound Rydberg electron with an electromagnetic half-cycle pulse (HCP) is described with the help of a multidimensional semiclassical treatment. This approach relates the quantum evolution of the electron to its…

Quantum Physics · Physics 2009-10-31 O. Zobay , G. Alber

A kick from a unipolar half-cycle pulse (HCP) can redistribute population and shift the relative phase between states in a radial Rydberg wave packet. We have measured the quantum coherence properties following the kick, and show that…

Quantum Physics · Physics 2009-11-10 J. M. Murray , S. N. Pisharody , H. Wen , P. H. Bucksbaum

Stark deceleration is a technique that uses time-varying inhomogeneous electric fields to decelerate polar molecules for various molecular beam and trapping experiments. New ring-geometry Stark decelerators with continuously varying…

Chemical Physics · Physics 2017-12-20 Yomay Shyur , Jason A. Bossert , H. J. Lewandowski

The dynamics of vibrational wave packets excited in K$_2$ dimers attached to superfluid helium nanodroplets is investigated by means of femtosecond pump-probe spectroscopy. The employed resonant three-photon-ionization scheme is studied in…

Atomic and Molecular Clusters · Physics 2009-11-11 P. Claas , G. Droppelmann , C. P. Schulz , M. Mudrich , F. Stienkemeier

The use of strong-field (i.e. intensities in excess of 10^13 Wcm-2) few-cycle ultrafast (durations of 10 femtoseconds or less) laser pulses to create, manipulate and image vibrational wavepackets is investigated. Quasi-classical modelling…

Chemical Physics · Physics 2017-02-08 W. A. Bryan , C. R. Calvert , R. B. King , J. B. Greenwood , W. R. Newell , I. D. Williams

We demonstrate an information hiding and retrieval scheme with the relative phases between states in a Rydberg wave packet acting as the bits of a data register. We use a terahertz half-cycle pulse (HCP) to transfer phase-encoded…

Quantum Physics · Physics 2009-11-13 J. M. Murray , S. N. Pisharody , H. Wen , C. Rangan , P. H. Bucksbaum

A partial-wave method is developed to deal with small molecules dominated by a central atom as an extension of earlier single-center methods. In particular, a model potential for the water molecule is expanded over a basis of spherical…

Chemical Physics · Physics 2022-04-06 Patrik Pirkola , Marko Horbatsch

The evolution of electron wavepackets determines the course of many physical and chemical phenomena and attosecond spectroscopy aims to measure and control such dynamics in real-time. Here, we investigate radial electron wavepacket motion…

Atomic Physics · Physics 2015-09-04 Niranjan Shivaram , Xiao-Min Tong , Henry Timmers , Arvinder Sandhu

In this paper a coherent superposition of angular momentum states created by absorption of polarized light by molecules is analyzed. Attention is paid to the time evolution of wave packets representing spatial orientation of internuclear…

Physics Education · Physics 2009-10-31 M. Auzinsh

SPEC_PULS describes a suite of computer programs to simulate the emergent spectrum from a radially-pulsating star. It combines a Christy-type non-linear pulsation code with classical stellar atmosphere codes. The principal aim is to…

Solar and Stellar Astrophysics · Physics 2022-06-29 C. Simon Jeffery

We investigate the time evolution of Gaussian wave packet (GWP) in the tight-binding chain with uniform nearest neighbor (NN) hopping integral. Analytical analysis and numerical simulations show that the fractional revival of the quantum…

Quantum Physics · Physics 2009-11-13 Bing Chen , Z. Song , C. P. Sun

The dynamics of vibrational wave packets excited in Na2 dimers in the triplet ground and excited states is investigated by means of helium nanodroplet isolation (HENDI) combined with femtosecond pump-probe spectroscopy. Different pathways…

Atomic and Molecular Clusters · Physics 2016-09-28 Patrick Claas , Georg Droppelmann , Claus-Peter Schulz , Marcel Mudrich , Frank Stienkemeier

We apply wave packet methods to study an ion-trap system in the strong excitation regime imposing neither the rotating wave nor the Lamb-Dicke approximations. By this approach we show the existence of states with restricted phase space…

Quantum Physics · Physics 2009-11-13 Dong Wang , Tony Hansson , Asa Larson , Hans O. Karlsson , Jonas Larson

We consider a model Hamiltonian describing the interaction of a single-mode radiation field with the atoms of a nonlinear medium, and study the dynamics of entanglement for specific non-entangled initial states of interest: namely, those in…

Quantum Physics · Physics 2007-07-01 C. Sudheesh , S. Lakshmibala , V. Balakrishnan

The coherent interaction with ultrashort light pulses is a powerful strategy for monitoring and controlling the dynamics of wave packets in all states of matter. As light presents an oscillation period of a few femtoseconds ($T=2.6$~fs in…

Stark deceleration allows for precise control over the velocity of a pulsed molecular beam and, by the nature of its limited phase-space acceptance, reduces the energy width of the decelerated packet. We describe an alternate method of…

Atomic Physics · Physics 2015-05-13 L. P. Parazzoli , N. Fitch , D. S. Lobser , H. J. Lewandowski

We present a theoretical analysis of the Stark effect in the hyperfine structure of the cesium ground-state. We have used third order perturbation theory, including diagonal and off-diagonal hyperfine interactions, and have identified terms…

Atomic Physics · Physics 2007-05-23 S. Ulzega , A. Hofer , P. Moroshkin , A. Weis

The semiclassical long-time limit of free evolution of quantum wave packets on the torus is under consideration. Despite of simplicity of this system, there are still open questions concerning the detailed description of the evolution on…

Quantum Physics · Physics 2017-06-28 A. S. Trushechkin

We observe the phase space trajectory of an entangled wave packet of a trapped ion with high precision. The application of a spin dependent light force on a superposition of spin states allows for coherent splitting of the matter wave…

Quantum Physics · Physics 2014-05-22 Ulrich Poschinger , Andreas Walther , Kilian Singer , Ferdinand Schmidt-Kaler

We investigate the response of two three-body Coulomb systems when driven by attosecond half-cycle pulses: The hydrogen molecular ion and the helium atom. Using very short half-cycle pulses (HCPs) which effectively deliver ``kicks'' to the…

Atomic Physics · Physics 2009-11-13 A. Emmanouilidou , T. Uzer
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