Related papers: Two-Photon Absorption
Two-photon absorption (TPA) and other nonlinear interactions of molecules with time-frequency-entangled photon pairs (EPP) has been predicted to display a variety of fascinating effects. Therefore, their potential use in practical…
We present a general theory to describe two-photon interference, including a formal description of few photon intereference in terms of single-photon amplitudes. With this formalism, it is possible to describe both frequency entangled and…
We theoretically investigate the two-photon absorption spectrum of conventional s-wave superconductors. The calculation is carried out in the local limit at absolute zero. The direct excitation of quasiparticles is excluded under the…
This paper presents an analysis of near-resonant, ro-vibrational two-photon spectroscopy and the use of cavity ring-down spectroscopy for its detection. Expressions are derived for the photon absorption rate of a three-level system, correct…
We have expressed the nonlinear optical absorption of a semiconductor in terms of its linear spectrum. We determined that the two-photon absorption coefficient in a strong DC-electric field of a direct gap semiconductor can be expressed as…
The position-representation wave function for multi-photon states and its equation of motion are introduced. A major strength of the theory is that it describes the complete evolution (including polarization and entanglement) of…
We demonstrate and study the enhancement of intermediate-field two-photon absorption by shaped femtosecond pulses having spectral phases of antisymmetric nature. The intermediate-field regime corresponds to pulse intensities, where the…
Rabi frequencies for multiphoton absorption by atoms or molecules that can be characterized as two- or three-level systems are obtained in the cases of single and double laser perturbations. If the ambiguity in the origin of absolute energy…
In order to obtain a classification of all possible quantum deformations of the two-photon algebra $h_6$, we introduce its corresponding general Lie bialgebra, which is a coboundary one. Two non-standard quantum deformations of $h_6$,…
We study the absorptive and dispersive properties of Doppler-broadened atomic media as a function of detuning. Beginning from the exact lineshape calculated for a two-level atom, a series of approximations to the electric susceptibility are…
Light transport in periodic waveguides coupled to a two-level atom is investigated. By using optical Bloch equations and a photonic modal formalism, we derive semi-analytical expressions for the scattering matrix of one atom trapped in a…
We consider theoretically nonlinear effects in a semiconductor quantum well embedded inside a photonic microcavity. Two-photon absorption by a 2p exciton state is considered and investigated; the matrix element of two-photon absorption is…
The purpose of this paper is to study the interaction between a two-level system and two continuous-mode photons. Two scenarios are investigated: Case 1, how a two-level system changes the pulse shapes of two input photons propagating in a…
Interaction of atoms with twisted light is the subject of intense experimental and theoretical investigation. In almost all studies, the atom is viewed as a localized probe of the twisted light field. However, as argued in this paper,…
Coherent control of femtosecond two-photon absorption in the intermediate-field regime is analyzed in detail in the powerful frequency domain using an extended 4th-order perturbative description. The corresponding absorption is coherently…
We evaluate the electric dipole absorption in small metal particles in a longitudinal electric field taking into account the Fermi-Thomas screening. When either the level broadening or the frequency of the field are larger than the mean…
We extend the powerful frequency-domain analysis of femtosecond two-photon absorption to the intermediate-field regime, which involves both two- and four-photon transitions. Consequently, we find a broad family of shaped pulses that enhance…
The nonlinear photon-photon interaction mediated by a single two-level atom is studied theoretically based on a one-dimensional model of the field-atom interaction. This model allows us to determine the effects of an atomic nonlinearity on…
The goal of this research is to determine and study a physical system that will enable a fast and intrinsically two-photon detector, which would be of interest for quantum information and metrology applications. We consider two types of…
We report on the dynamics of photodegradation and subsequent recovery of two-photon fluorescence in a dye-doped polymer. The energy dependence suggests that photo-degradation is a linear process while recovery is entropic. Such recovery…