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The motion of electrons and ions in medium-sized rare gas clusters (1000 atoms) exposed to intense laser pulses is studied microscopically by means of classical molecular dynamics using a hierarchical tree code. Pulse parameters for optimum…

Atomic and Molecular Clusters · Physics 2007-05-23 Ulf Saalmann , Jan-Michael Rost

We have developed a perturbative method to model the resonant ionization of atomic systems in fluctuating laser fields. The perturbative method is based on an expansion in terms of the multitime cumulants, a suitable combination of moments…

Atomic Physics · Physics 2020-11-25 Tejaswi Katravulapally , L. A. A. Nikolopoulos

We present a general variational approach for computing the laser-induced rovibrational dynamics of molecules taking into account the hyperfine effects of the nuclear quadrupole coupling. The method combines the general variational approach…

Atomic and Molecular Clusters · Physics 2020-06-18 Andrey Yachmenev , Linda V. Thesing , Jochen Küpper

We present extensive molecular dynamics simulations of a liquid of symmetric dumbbells, for constant packing fraction, as a function of temperature and molecular elongation. For large elongations, translational and rotational degrees of…

Soft Condensed Matter · Physics 2009-11-11 Angel J. Moreno , Song-Ho Chong , Walter Kob , Francesco Sciortino

We theoretically investigate the generation of ultrafast currents in insulators induced by strong few-cycle laser pulses. Ab initio simulations based on time-dependent density functional theory give insight into the atomic-scale properties…

After the clasical approach to acceleration of a charged particle by delta-form impulsive force, we consider the corresponding quantum theory based on the Volkov solution of the Dirac equation. We determine the modified Compton formula for…

High Energy Physics - Phenomenology · Physics 2007-05-23 Miroslav Pardy

Time-dependent coupled-cluster method with time-varying orbital functions, called time-dependent optimized coupled- cluster (TD-OCC) method, is formulated for multielectron dynamics in an intense laser field. We have successfully derived…

Chemical Physics · Physics 2018-03-14 Takeshi Sato , Himadri Pathak , Yuki Orimo , Kenichi L. Ishikawa

Circularly-polarized light is well-known to induce, or flip the direction of, magnetization in solids. At its heart, this arises from time-reversal symmetry breaking by the vector potential, causing inverse-Faraday or analogous physical…

Optics · Physics 2025-07-22 Ofer Neufeld

The generation of laser-driven dense relativistic electron layers from ultra-thin foils and their use for coherent Thomson backscattering is discussed, applying analytic theory and one-dimensional particle-in-cell simulation. The blow-out…

Plasma Physics · Physics 2009-11-13 Jürgen Meyer-ter-Vehn , Hui-Chun Wu

Particle-in-cell codes are now standard tools for studying ultra-intense laser-plasma interactions. Motivated by direct laser acceleration of electrons in sub-critical plasmas, we examine temporal resolution requirements that must be…

This paper concerns the theory of non-recollisional ionization or detachment of atoms or ions by intense few-cycle pulses. It is shown that in certain conditions of pulse duration, peak intensity and carrier-envelope phase, the ionization…

Atomic Physics · Physics 2014-09-04 C. C. Chirila , R. M. Potvliege

Ultrashort laser pulses pose unique tools to trigger and probe the fastest charge dynamics in matter, allowing the investigation of fundamental physical phenomena with unprecedented resolution in space, time, and energy. One of the most…

Optics · Physics 2025-03-27 Dino Habibović , Kathryn R. Hamilton , Ofer Neufeld , Laura Rego

We show that field-free molecular orientation induced by a half-cycle pulse may be considerably enhanced by an additional laser pulse inducing molecular anti-alignment. Two qualitatively different enhancement mechanisms are identified…

Quantum Physics · Physics 2009-11-11 E. Gershnabel , I. Sh. Averbukh , R. J. Gordon

We identify that both the dynamic core polarization and dynamic orbital deformation are important in the orientation-dependent high-harmonic generation of CO molecules subjected to intense few cycle laser fields. These polarization dynamics…

Atomic Physics · Physics 2015-06-19 Bin Zhang , Jianmin Yuan , Zengxiu Zhao

Ultrafast laser pulse has provided a systematic way to inspect the dynamics of electrons in condensed matter systems. In this paper, by means of time-dependent density matrix renormalization group, we study an ultrafast laser driven Kondo…

Strongly Correlated Electrons · Physics 2021-06-23 W. Zhu , Benedikt Fauseweh , Alexis Chacon , Jian-Xin Zhu

The ability to directly follow and time resolve the rearrangement of the nuclei within molecules is a frontier of science that requires atomic spatial and few-femtosecond temporal resolutions. While laser induced electron diffraction can…

Models which allow an explicit application to structurally modulated substances are reviewed within the frame of a symmetry-based approach starting from discrete lattice theory. Focus is set on models formulated in terms of local variables…

Condensed Matter · Physics 2007-05-23 Boris Neubert , Michel Pleimling , Rolf Siems

We have developed a variational perturbation theory based on the Liouville-Neumann equation, which enables one to systematically compute the perturbative correction terms to the variationally determined wave functions of the time-dependent…

High Energy Physics - Theory · Physics 2008-11-26 Dongsu Bak , Sang Pyo Kim , Sung Ku Kim , Kwang-Sup Soh , Jae Hyung Yee

Alignment and orientation of molecules by intense, ultrashort laser fields are crucial for a variety of applications in physics and chemistry. These include control of high harmonics generation, molecular orbitals tomography, control of…

We report a theoretical study of the optical centrifuge acceleration of an asymmetric top molecule interacting with an electric static field by solving the time-dependent Schr\"odinger equation in the rigid rotor approximation. A detailed…

Chemical Physics · Physics 2018-02-14 Juan J. Omiste