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We studied intensity fluctuations of a single photon source relying on the pulsed excitation of the fluorescence of a single molecule at room temperature. We directly measured the Mandel parameter Q(T) over 4 orders of magnitude of…

Quantum Physics · Physics 2009-11-07 F. Treussart , R. Alleaume , V. Le Floc'h , L. T. Xiao , J. -M Courty , J. -F. Roch

Single-photon sources are a fundamental resource in quantum optics. The indistinguishability and purity of photons emitted from different sources are crucial (necessary, essential) properties for many quantum applications to ensure…

Quantum Physics · Physics 2020-07-15 Valérian Thiel , Alex O. C. Davis , Ke Sun , Peru D'Ornellas , Xian-Min Jin , Brian J. Smith

Mandel Q-parameter, which is determined from single event photon statistics, provides an alternative to differentiate single-molecule with fluorescence detection. In this work, by using the Q-parameter of the sample fluorescence compared to…

Quantum Physics · Physics 2009-11-13 Shuangli Dong , Tao Huang , Yuan Liu , Jun Wang , Guofeng Zhang , Liantuan Xiao+ , Suotang Jia

We present a general relation between Mandel's $Q$ parameter describing variance of number of photons emitted from a single molecule and a three time correlation function describing a spectral diffusion process the molecule is undergoing.…

Statistical Mechanics · Physics 2007-05-23 Eli Barkai , YounJoon Jung , Robert Silbey

We derive the moment generating function for photon emissions from a single molecule driven by laser excitation. The frequencies of the fluoresced photons are explicitly considered. Calculations are performed for the case of a two level dye…

Statistical Mechanics · Physics 2009-08-14 Golan Bel , Frank L. Brown

A theory is formulated for time dependent fluctuations of the spectrum of a single molecule in a dynamic environment. In particular, we investigate the photon counting statistics of a single molecule undergoing a spectral diffusion process.…

Statistical Mechanics · Physics 2007-05-23 YounJoon Jung , Eli Barkai , Robert J. Silbey

A promising result from optical quantum metrology is the ability to achieve sub-shot-noise performance in transmission or absorption measurements. This is due to the significantly lower uncertainty in light intensity of quantum beams with…

Quantum Physics · Physics 2021-09-01 Agustina G. Magnoni , Laura T. Knoll , Miguel A. Larotonda

Through examining the product of the mathematical variance of intensity with respect to time and frequency, we arrive at a temporal characterization of laser pulses through parameters for pulse duration, group delay dispersion and temporal…

Single-photon sources are at the heart of quantum-optical networks, with their uniquely quantum emission and phenomenon of two-photon interference allowing for the generation and transfer of nonclassical states. Although a few analytical…

Quantum Physics · Physics 2018-02-08 Kevin A. Fischer , Kai Müller , Konstantinos G. Lagoudakis , Jelena Vučković

A central challenge in computational modeling of dynamic biological systems is parameter inference from experimental time course measurements. However, one would not only like to infer kinetic parameters but also study their variability…

A simple model system is introduced for demonstrating how a single photon source might be used to transduce classical analog information. The theoretical scheme results in measurements of analog source samples that are (i) quantized in the…

Quantum Physics · Physics 2016-09-26 Mark D. McDonnell , Adrian P. Flitney

We demonstrate by time-resolved resonance fluorescence measurements on a single self-assembled quantum dot an internal photo-effect that emits electrons from the dot by an intra-band excitation. We find a linear dependence of the optically…

Mesoscale and Nanoscale Physics · Physics 2021-02-24 Pia Lochner , Jens Kerski , Annika Kurzmann , Andreas D. Wieck , Arne Ludwig , Martin Geller , Axel Lorke

Estimating the quality of a single-photon source is crucial for its use in quantum technologies. The standard test for semiconductor sources is a value of the second-order correlation function of the emitted field below $1/2$ at zero…

Quantum Physics · Physics 2020-05-12 Jorge Rolando Chavez-Mackay , Peter Grünwald , Blas Manuel Rodríguez-Lara

Suppose we measure the time-dependent spectrum of a single photon. That is, we first send the photon through a set of frequency filters (which we assume to have different filter frequencies but the same finite bandwidth $\Gamma$), and then…

Quantum Physics · Physics 2017-09-27 S. J. van Enk

We present a method to classically enhance noise-robustness of single-pixel imaging in photon counting regime with a pulsed source. By using time-domain cross-correlations between temporal profiles of a pulsed source and received signals,…

We study a quantum-enhanced differential measurement scheme that uses quantum probes and single-photon detectors to measure a minute defect in the absorption parameter of an analyte under investigation. For the purpose, we consider two…

Quantum Physics · Physics 2022-04-07 Byeong-Yoon Go , Changhyoup Lee , Kwang-Geol Lee

Measuring the power spectral density of a stochastic process, such as a stochastic force or magnetic field, is a fundamental task in many sensing applications. Quantum noise is becoming a major limiting factor to such a task in future…

Intensity interferometry is a well known method in astronomy. Recently, a related method called incoherent diffractive imaging (IDI) was proposed to apply intensity correlations of x-ray fluorescence radiation to determine the 3D…

Optics · Physics 2020-08-27 Fabian Trost , Kartik Ayyer , Henry Chapman

For near-term quantum devices, an important challenge is to develop efficient methods to certify that noise levels are low enough to allow potentially useful applications to be carried out. We present such a method tailored to photonic…

Quantum Physics · Physics 2022-02-11 Rawad Mezher , Shane Mansfield

Variable-intensity astronomical sources are the result of complex and often extreme physical processes. Abrupt changes in source intensity are typically accompanied by equally sudden spectral shifts, i.e., sudden changes in the wavelength…

Applications · Statistics 2015-12-14 Raymond K. W. Wong , Vinay L. Kashyap , Thomas C. M. Lee , David A. van Dyk
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