Related papers: Preparing high purity initial states for nuclear m…

Nuclear magnetic resonance spectroscopy is one of the few remaining areas of physical chemistry for which polynomially scaling simulation methods have not so far been available. Here, we report such a method and illustrate its performance…

We discuss the use of a region of uniform and constant magnetic field in order to implement a two-state atomic polarizer for an H(2S) beam. We have observed that a device with such field configuration is capable of achieving an efficient…

Manipulation of solid-state spin coherence is an important paradigm for quantum information processing. Current systems either operate at very low temperatures or are difficult to scale-up. Developing low-cost, scalable materials whose…

We report the structural transformation of hexagonal Ba3YIr2O9 to a cubic double perovskite form (stable in ambient conditions) under an applied pressure of 8GPa at 1273K. While the ambient pressure (AP) synthesized sample undergoes…

This paper shows how the Greenberger-Horne-Zeilinger experiment, which demonstrates the nonlocal nature of quantum mechanics, can be performed using nuclear magnetic resonance on spins in molecules at finite temperature. The use of nuclear…

We propose a novel MRI (Magnetic Resonance Imaging) technique based quantum bit (qubit) generation with water proton NMR (1H-NMR), distinct from previously proposed NMR chemical shift or spectroscopic techniques based qubit generation. We…

Quantum state readout is a key requirement for a successful qubit platform. In this work we demonstrate a high fidelity quantum state readout of a V2 center nuclear spin based on a repetitive readout technique. We demonstrate up to…

We report the first use of "logical labeling" to perform a quantum computation with a room-temperature bulk system. This method entails the selection of a subsystem which behaves as if it were at zero temperature - except for a decrease in…

We propose a new approach to the measurement of a single spin state, based on nuclear magnetic resonance (NMR) techniques and inspired by the coherent control over many-body systems envisaged by Quantum Information Processing (QIP). A…

The ability to control and exploit quantum coherence and entanglement drives research across many fields ranging from ultra-cold quantum gases to spin systems in condensed matter. Transcending different physical systems, optical approaches…

We derive a general formula for the paramagnetic NMR nuclear shielding tensor of an open-shell molecule in a pure spin state, subject to a zero-field splitting (ZFS). Our findings are in contradiction with a previous proposal. We present a…

For applications of solid state quantum computing and quantum simulations, high fidelity initialisation of thermally mixed electronic and nuclear spin qubits is essential. Whereas electronic spins can readily be initialised optically to…

The nuclear spin is a prime candidate for quantum information applications due to its weak coupling to the environment and inherently long coherence times. However, this weak coupling also challenges the addressability of the nuclear spin.…

A three-qubit 13C solid-state nuclear magnetic resonance (NMR) system for quantum information processing, based on the malonic acid molecule, is used to demonstrate high-fidelity universal quantum control via strongly-modulating…

We study the nuclear spin population in a GaAs quantum well structure and demonstrate its initialization using an all-electrical nuclear magnetic resonance (NMR) device. In our device, nuclear spins are dynamically polarized in a sub-micron…

Using the concept of the so-called quantum relaxation, we build a semiphenomenological model for orto-para conversion of nuclear spin isomers of hydrogen-type molecules.

We investigate analytically and numerically the Multiple Quantum (MQ) NMR dynamics in systems of nuclear spins 1/2 coupled by the dipole-dipole interactions in the case of the dipolar ordered initial state. We suggest two different methods…

We employ a quantum computer to simulate the effect of spin impurities on nitrogen-vacancy (NV) centers in diamond. As these defects operate as nanoscale quantum sensors, modeling quantum noise is crucial to identify limitations in…

In this work, we experimentally demonstrate the implementation of a recently proposed robust and state-independent heat-bath algorithmic cooling (HBAC) method [1] on an NMR quantum processor. While HBAC methods improve the purity of a…

The hyperpolarisation of nuclear spins within target molecules is a critical and complex challenge in magnetic resonance imaging (MRI) and nuclear magnetic resonance (NMR) spectroscopy. Hyperpolarisation offers enormous gains in signal and…