Related papers: Reaching optimally oriented molecular states by la…
The generation of ultrashort pulses hinges on the careful management of dispersion. Traditionally, this has exclusively involved second-order dispersion, while higher-order dispersion was treated as a nuisance to be minimized. Here we show…
The transition between two distinct mechanisms for the laser-induced field-free orientation of CO molecules is observed via measurements of orientation revival times and subsequent comparison to theoretical calculations. In the first…
Scattering of ultraintense short laser pulses off relativistic electrons allows one to generate a large number of X- or $\gamma$-ray photons with the expense of the spectral width---temporal pulsing of the laser inevitable leads to…
We demonstrate experimentally a method of varying the degree of directionality in laser-induced molecular rotation. To control the ratio between the number of clockwise and counter-clockwise rotating molecules (with respect to a fixed…
We demonstrate for the first time that a matter physical two level system, a qubit, can be fully controlled using one ultrafast step. We show that the spin state of an optically excited electron, an exciton, confined in a quantum dot, can…
We study the dynamics of multipulse solutions in mode-locked lasers in presence of time-delayed feedback stemming, e.g., from reflections upon optical elements, and carrier dynamics. We demonstrate that the dynamics of such a high…
Laser-driven ion acceleration from nanostructured targets offers a promising route to compact, high-energy ion sources. In this work, we demonstrate through particle-in-cell simulations that rectangular nanoring targets significantly…
Preparation of a so-called circular state in a Rydberg atom where the projection of the electron angular momentum takes its maximum value is challenging due to the required amount of angular momentum transfer. Currently available protocols…
We study the possibility of efficient self-compression of femtosecond laser pulses in nonlinear media with anomalous dispersion of group velocity during the self-focusing of wave packets with a power several times greater than the critical…
We present the results of theoretical studies on operations with charge qubits in the system composed of two tunnel-coupled semiconductor quantum dots whose two lowest states (localized in different dots) define the logical qubit states…
Most quantum processors requires pulse sequences for controlling quantum states. Here, we present an alternative algorithm for computing an optimal pulse sequence in order to perform a specific task, being an implementation of a quantum…
Two dimensional particle-in-cell simulations characterizing the interaction of ultraintense short pulse lasers in the range 10^{18} \leq I \leq 10^{20} W/cm^{2} with converging target geometries are presented. Seeking to examine intensity…
We investigate to which extend a THz laser pulse can be used to produce field-free molecular orientation at high temperature. We consider laser pulses that can be implemented with the state of the art technology and we show that the…
Inducing and controlling the ultrafast molecular rotational dynamics using shaped laser fields is essential in numerous applications. Several approaches exist that allow following the coherent molecular motion in real-time, including…
Globally optimal solution describing a phase conjugated field of Raman scattering on the resonant $B\gets X$ transition of iodine $I_2$ is studied. Maximum optical coherence is found as a top eigenvalue problem. A reversibility theorem has…
We formulate a novel planar motion planning problem for a Dubins-Laser system that consists of a Dubins vehicle with an attached controllable laser. The vehicle moves with unit speed and the laser, having a finite range, can rotate in a…
Enantioselective orientation of chiral molecules excited by a shaped picosecond laser pulse and a delayed femtosecond pulse is considered. Using quantum mechanical simulations, we demonstrate a strong field-free enantioselective orientation…
In this article we analyze the optimal control strategy for rotating a monitored qubit from an initial pure state to an orthogonal state in minimum time. This strategy is described for two different cost functions of interest which do not…
We produce oriented rotational wave packets in CO and measure their characteristics via high harmonic generation. The wavepacket is created using an intense, femtosecond laser pulse and its second harmonic. A delayed 800 nm pulse probes the…
We demonstrate experimentally a method of all-optical selective rotational control in gas mixtures. Using an optical centrifuge - an intense laser pulse whose linear polarization rotates at an accelerated rate, we simultaneously excite two…