Related papers: Rotational master equation for cold laser-driven m…
Collective states in cold nuclei are represented by a wave function that assigns coherent phases to the participating nucleons. The degree of coherence decreases with excitation energy above the yrast line because of coupling to the…
We apply two different monotonically convergent optimization algorithms to the control of molecular rotational dynamics by laser pulses. This example represents a quantum control problem where the interaction of the system with the external…
We consider a molecular aggregate consisting of $N$ identical monomers. Each monomer comprises two electronic levels and a single harmonic mode. The monomers interact with each other via dipole-dipole forces. The monomer vibrational modes…
The angular momentum of molecules, or, equivalently, their rotation in three-dimensional space, is ideally suited for quantum control. Molecular angular momentum is naturally quantized, time evolution is governed by a well-known Hamiltonian…
Levitated nanoparticles are a promising platform for sensing applications and for macroscopic quantum experiments. While the nanoparticles' motional temperatures can be reduced to near absolute zero, their uncontrolled internal degrees of…
We show that quantum rotational wavepacket dynamics in molecules can be described by a new system-environment model, which consists of a rotational subsystem coupled to a magnetically tunable spin bath formed by the nuclear spins within the…
Conventional techniques for laser cooling, by coherent scattering off of internal states or through an optical cavity mode, have so far proved inefficient on mechanical oscillators heavier than a few nanograms. That is because larger…
We present detailed calculations at the basis of our recent proposal for simultaneous cooling the rotational, vibrational and external molecular degrees of freedom. In this method, the molecular rovibronic states are coupled by an intense…
We examine the potential-energy curves and polarization of the dipole moments of two static polar molecules under the influence of an external dc electric field and their anisotropic dipole-dipole interaction. We model the molecules as…
Within the framework of master equation, we study decay dynamics of an atom-molecule system strongly coupled by two photoassociation lasers. Summing over the infinite number of electromagnetic vacuum modes that are coupled to the…
We predict that it is possible to cool rotational, vibrational and translational degrees of freedom of molecules by coupling a molecular dipole transition to an optical cavity. The dynamics is numerically simulated for a realistic set of…
A fascinating effect belonging to the field of vacuum forces and fluctuations is that of quantum friction. It refers to the prediction of a dissipative force acting on a moving object due to the quantum vacuum field. In this work, we…
Atoms trapped in a red detuned retro-reflected Laguerre-Gaussian beam undergo orbital motion within rings whose centers are on the axis of the laser beam. We determine the wave functions, energies and degeneracies of such quantum rotors…
The effect of decoherence, induced by spontaneous emission, on the dynamics of cold atoms periodically kicked by an optical lattice is experimentally and theoretically studied. Ideally, the mean energy growth is essentially unaffected by…
Laser cycling of resonances can remove entropy from a system via spontaneously emitted photons, with electronic resonances providing the fastest cooling timescales because of their rapid relaxation rates. Although atoms are routinely laser…
Laser control of molecular rotation is an area of active research. A number of recent studies has aimed at expanding the reach of rotational control to extreme, previously inaccessible rotational states, as well as controlling the…
Memory effects in open quantum dynamics are often incorporated in the equation of motion through a superoperator known as the memory kernel, which encodes how past states affect future dynamics. However, the usual prescription for…
The formation of diatomic molecules with rotational and vibrational coherence is demonstrated experimentally in free-to-bound two-photon femtosecond photoassociation of hot atoms. In a thermal gas at a temperature of 1000 K, pairs of…
We give a detailed derivation of the master equation description of the coherent backscattering of laser light by cold atoms. In particular, our formalism accounts for the nonperturbative nonlinear response of the atoms when the injected…
We analytically derive the exact -- though formal -- master equation for a two-level quantum system (qubit) interacting with a bosonic environment within the rotating-wave approximation, assuming the environment is initially in an arbitrary…