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Molecular spins are promising candidates for quantum information science, leveraging coherent electronic spin states for quantum sensing and computation. However, the practical application of these systems is hindered by electronic spin…

Quantum Physics · Physics 2026-03-03 Timothy J. Krogmeier , Anthony W. Schlimgen , Kade Head-Marsden

Mapping the system evolution of a two-state system allows the determination of the effective system Hamiltonian directly. We show how this can be achieved even if the system is decohering appreciably over the observation time. A method to…

We present and test a new algorithm for time-evolving quantum many-body systems initially proposed by Holzner et al. [Phys. Rev. B 83, 195115 (2011)]. The approach is based on merging the matrix product state (MPS) formalism with the method…

Strongly Correlated Electrons · Physics 2018-07-23 Jad C. Halimeh , Fabian Kolley , Ian P. McCulloch

In many realizations of electron spin qubits the dominant source of decoherence is the fluctuating nuclear spin bath of the host material. The slowness of this bath lends itself to a promising mitigation strategy where the nuclear spin bath…

Mesoscale and Nanoscale Physics · Physics 2010-11-30 Hendrik Bluhm , Sandra Foletti , Diana Mahalu , Vladimir Umansky , Amir Yacoby

The dynamics of a qubit under the decoherence of a two level fluctuator (TLF) in addition to its coupling to a bosonic bath is investigated theoretically. Two different methods are applied and compared for this problem. One is a…

Quantum Physics · Physics 2010-11-12 Peihao Huang , Hang Zheng , Keiichiro Nasu

We introduce, and determine decoherence for, a wide class of non-trivial quantum spin baths which embrace Ising, XY and Heisenberg universality classes coupled to a two-level system. For the XY and Ising universality classes we provide an…

We propose a new approach to simulate the decoherence of a central spin coupled to an interacting dissipative spin bath with cluster-correlation expansion techniques. We benchmark the approach on generic 1D and 2D spin baths and find…

Quantum Physics · Physics 2023-12-05 Mykyta Onizhuk , Yu-Xin Wang , Jonah Nagura , Aashish A. Clerk , Giulia Galli

Decoherence of a central spin coupled to an interacting spin bath via inhomogeneous Heisenberg coupling is studied by two different approaches, namely an exact equations of motion (EOMs) method and a Chebyshev expansion technique (CET). By…

Mesoscale and Nanoscale Physics · Physics 2016-01-20 Ning Wu , Nina Fröhling , Xi Xing , Johannes Hackmann , Arun Nanduri , Frithjof B. Anders , Herschel Rabitz

We use the "generalized hierarchical equation of motion" proposed in Paper I to study decoherence in a system coupled to a spin bath. The present methodology allows a systematic incorporation of higher order anharmonic effects of the bath…

Chemical Physics · Physics 2018-01-17 Chang-Yu Hsieh , Jianshu Cao

We present a perturbative treatment of the subohmic spin-boson model which remedies a crucial flaw in previous treatments. The problem is traced back to the incorrect application of a Markov type approximation to specific terms in the…

Mesoscale and Nanoscale Physics · Physics 2014-12-10 Kyung-Joo Noh , Uwe R. Fischer

Using Suzuki-Trotter decompositions of exponential operators we describe new algorithms for the numerical integration of the equations of motion for classical spin systems. These techniques conserve spin length exactly and, in special…

Statistical Mechanics · Physics 2015-06-25 D. P. Landau , Shan-Ho Tsai , M. Krech , Alex Bunker

A perfect quantum state transfer(QST) has been shown in an engineered spin chain with "always-on interaction". Here, we consider a more realistic problem for such a protocol, the quantum decoherence induced by a spatially distributed…

Quantum Physics · Physics 2007-05-23 Lan Zhou , Jing Lu , Tao Shi , C. P. Sun

We investigate the decoherence properties of a central system composed of two spins 1/2 in contact with a spin bath. The dynamical regime of the bath ranges from a fully integrable integrable limit to complete chaoticity. We show that the…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 A. Relano , J. Dukelsky , R. A. Molina

Decoherence of electron spins in nanoscale systems is important to quantum technologies such as quantum information processing and magnetometry. It is also an ideal model problem for studying the crossover between quantum and classical…

Mesoscale and Nanoscale Physics · Physics 2017-03-06 Wen Yang , Wen-Long Ma , Ren-Bao Liu

We demonstrate through exact solutions that a spin bath leads to stronger (faster) dephasing of a qubit than a bosonic bath with identical bath-coupling spectrum. This difference is due to the spin-bath "dressing" by the coupling.…

Quantum Physics · Physics 2011-06-10 D. D. Bhaktavatsala Rao , Gershon Kurizki

Spin decoherence poses a significant challenge in molecular magnets, with the nuclear spin bath serving as a prominent source. Intriguingly, spin qubits at the clock transition exhibit remarkable insensitivity to the surrounding nuclear…

Quantum Physics · Physics 2025-10-14 Xiao Chen , Haechan Park , Silas Hoffman , Shuanglong Liu , Hai-Ping Cheng

Unwanted interaction between a quantum system and its fluctuating environment leads to decoherence and is the primary obstacle to establishing a scalable quantum information processing architecture. Strategies such as environmental and…

Decoherence of a center spin or qubit in a spin bath is essentially determined by the many-body bath evolution. We develop a cluster-correlation expansion (CCE) theory for the spin bath dynamics relevant to the qubit decoherence problem. A…

Mesoscale and Nanoscale Physics · Physics 2008-08-25 Wen Yang , Ren-bao Liu

We present an approach that allows quantifying decoherence processes in an open quantum system subject to external time-dependent control. Interactions with the environment are modeled by a standard bosonic heat bath. We develop two…

Mesoscale and Nanoscale Physics · Physics 2010-10-12 Dmitry Solenov , Vladimir Privman

We develop a mathematical description of the decoherence caused by "spin baths", such as nuclear spins or magnetic impurities. In contrast to the usual oscillator bath models of quantum environments, decoherence in the spin bath can occur…

Condensed Matter · Physics 2007-05-23 N. V. Prokof'ev , P. C. E. Stamp