Related papers: Direct Measurement of the Photon Statistics of a T…
n a recent experiment, we reported the time-domain intensity noise measurement of a single photon source relying on single molecule fluorescence control. In this article we present data processing, starting from photocount timestamps. The…
We derive the moment generating function for photon emissions from a single molecule driven by laser excitation. The frequencies of the fluoresced photons are explicitly considered. Calculations are performed for the case of a two level dye…
Mandel Q-parameter, which is determined from single event photon statistics, provides an alternative to differentiate single-molecule with fluorescence detection. In this work, by using the Q-parameter of the sample fluorescence compared to…
A theory is formulated for time dependent fluctuations of the spectrum of a single molecule in a dynamic environment. In particular, we investigate the photon counting statistics of a single molecule undergoing a spectral diffusion process.…
Through examining the product of the mathematical variance of intensity with respect to time and frequency, we arrive at a temporal characterization of laser pulses through parameters for pulse duration, group delay dispersion and temporal…
Shot noise sets a fundamental limit on the sensitivity of classical optical measurements, with coherent emitters achieving the lowest possible shot-noise level. Emission from sub-Poissonian light provides a pathway to surpass this limit,…
A two-level atom cannot emit more than one photon at a time. As early as the 1980s, this quantum feature was identified as a gateway to "single-photon sources", where a regular excitation sequence would create a stream of light particles…
Intensity squeezing, i.e., photon number fluctuations below the shot noise limit, is a fundamental aspect of quantum optics and has wide applications in quantum metrology. It was predicted in 1979 that the intensity squeezing could be…
Single-photon sources are a fundamental resource in quantum optics. The indistinguishability and purity of photons emitted from different sources are crucial (necessary, essential) properties for many quantum applications to ensure…
We demonstrate a single-photon source based on a quantum dot in a micropost microcavity that exhibits a large Purcell factor together with a small multi-photon probability. For a quantum dot on resonance with the cavity, the spontaneous…
A pulsed source of entangled photons is desirable for some applications. Yet, such a source has intrinsic problems arising from the simultaneous arrival of the signal and noise photons to the detectors. These problems are analyzed and…
We present a general relation between Mandel's $Q$ parameter describing variance of number of photons emitted from a single molecule and a three time correlation function describing a spectral diffusion process the molecule is undergoing.…
The fluorescence of a single dipole excited by an intense light pulse can lead to the generation of another light pulse containing a single photon. The influence of the duration and energy of the excitation pulse on the number of photons in…
Single dye molecules at cryogenic temperatures display many spectroscopic phenomena known from free atoms and are thus promising candidates for fundamental quantum optical studies. However, the existing techniques for the detection of…
Photon number distributions from classical and non-classical light sources have been studied extensively, yet their impact on photoemission processes is largely unexplored. In this article, we present measurements of electron…
We investigate the photon statistics of a single-photon source that operates under non-stationary conditions. The photons are emitted by shining a periodic sequence of laser pulses on single atoms falling randomly through a high-finesse…
We investigate the intensity correlation properties of single photons emitted from an optically excited single semiconductor quantum dot. The second order temporal coherence function of the photons emitted at various wavelengths is measured…
The construction of a single photon source using gated parametric fluorescence is reported with the measurement results of the photon number distribution. A beamlike twin-photon method is used in order to achieve high collection efficiency.…
Single-photon sources are at the heart of quantum-optical networks, with their uniquely quantum emission and phenomenon of two-photon interference allowing for the generation and transfer of nonclassical states. Although a few analytical…
It has been observed experimentally [H.R. Xia, C.Y. Ye, and S.Y. Zhu, Phys. Rev. Lett. {\bf 77}, 1032 (1996)] that quantum interference between two molecular transitions can lead to a suppression or enhancement of spontaneous emission. This…