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We consider the generation of microscopic polarization in two-dimensional semiconductors under intense optical fields in the nonresonant regime. We demonstrate that the intraband motion of quasiparticles, driven by the electric field of the…

Mesoscale and Nanoscale Physics · Physics 2025-01-14 A. O. Slobodeniuk , T. Novotný

We make use of an inhomogeneous electrostatic dipole field to impart a quantum-state-dependent deflection to a pulsed beam of OCS molecules, and show that those molecules residing in the absolute ground state, $X ^1\Sigma^+$, $\ket{00^00}$,…

The amplitude and probability of quantum transitions are represented as a path integrals in energy state space of the investigated multi-level quantum system. Using this approach we consider rotational dynamics of nitrogen molecules…

Quantum Physics · Physics 2014-07-16 Alexander Biryukov , Mark Shleenkov

Using the Brink-Axel hypothesis we derive the rate $R$ for nuclear dipole excitation by a laser pulse carrying $N \gg 1$ photons with average energy $\hbar \omega_0 \approx 5$ MeV. As expected $R \propto (\hbar \omega_0)^3$. The rate is…

Nuclear Theory · Physics 2020-05-06 Adriana Pálffy , Paul-Gerhard Reinhard , Hans A. Weidenmüller

A comprehensive theoretical approach to describe the electron-ion radiative recombination in the presence of intense, short laser pulses, which accounts for nondipole corrections is presented. It is based on the relativistic Coulomb-Volkov…

Quantum Physics · Physics 2024-05-13 Deeksha Kanti , M. M. Majczak , J. Z. Kamiński , Liang-You Peng , K. Krajewska

Plasma dipole oscillation (PDO) depicted as harmonic motion of a spatially localized block of electrons has, until now, been hypothetical. In practice, the plasma oscillation occurs always as a part of a plasma wave. Studies on radiation…

A new numerical method is introduced for calculating the polarizability of an arbitrary dielectric object with position dependent complex permittivity. Three separate numerical approaches are provided to calculate the dipole moment of a…

Materials Science · Physics 2022-03-18 Daniel B. Murray , Caleb H. Netting , Robin D. Mercer , Lucien Saviot

D$_2$ molecules, excited by linearly cross-polarized femtosecond extreme ultraviolet (XUV) and near-infrared (NIR) light pulses, reveal highly structured D$^+$ ion fragment momenta and angular distributions that originate from two different…

CO$_2$ dissociation stimulated by vibrational excitation in non-equilibrium discharges has drawn lots of attention. Ns-discharges are known for their highly non-equilibrium conditions. It is therefore of interest to investigate the CO$_2$…

Plasma Physics · Physics 2021-07-02 Yanjun Du , Tsanko V. Tsankov , Dirk Luggenhölscher , Uwe Czarnetzki

Traditional theories of the NMR autocorrelation function for intramolecular dipole pairs assume single-exponential decay, yet the calculated autocorrelation of realistic systems display a rich, multi-exponential behavior resulting in…

We present a theoretical study of the rotational dynamics of asymmetry top molecules in an electric field and a parallel non-resonant linearly polarized laser pulse. The time-dependent Schr\"odinger equation is solved within the rigid rotor…

Quantum Physics · Physics 2015-06-16 Juan J. Omiste , Rosario González-Férez

Quantum molecular dynamics requires an accurate representation of the molecular potential energy surface from a minimal number of electronic structure calculations, particularly for nonadiabatic dynamics where excited states are required.…

Chemical Physics · Physics 2016-08-24 Charles W. Heaps , David A. Mazziotti

The propagation and scattering of electromagnetic waves in magnetized plasmas in a state where a global mode has been established or is in turbulence, are of theoretical and experimental interest in thermonuclear fusion research.…

A theoretical comparison of the electronic excitation and ionisation behaviour of molecular hydrogen oriented either parallel or perpendicular to a linear polarised laser pulse is performed. The investigation is based on a non-perturbative…

Quantum Physics · Physics 2009-11-13 Yulian V. Vanne , Alejandro Saenz

The formation of pulses of surface electromagnetic waves in a metal/dielectric interface is considered in the process of cooperative decay of excitons of quantum dots distributed near a metal surface in a dielectric layer. It is shown that…

Mesoscale and Nanoscale Physics · Physics 2017-03-08 A. V. Shesterikov , M. Yu. Gubin , M. G. Gladush , A. Yu. Leksin , A. V. Prokhorov

To solve the time-dependent Schr\"odinger equation in spatially inhomogeneous pulses of electromagnetic radiation, we propose an iterative semi-classical complex trajectory approach. In numerical applications, we validate this method…

Atomic and Molecular Clusters · Physics 2020-01-29 Jianxiong Li , Uwe Thumm

We show how one can perform arbitrary rotation of any qubit, using delayed laser pulses through nonadiabatic evolution, i.e., via transitions among the adiabatic states. We use a double-Lambda scheme and use a set of control parameters such…

Quantum Physics · Physics 2007-05-23 Asoka Biswas , G. S. Agarwal

A general {\it ab-initio} and non-perturbative method to solve the time-dependent Schr\"odinger equation (TDSE) for the interaction of a strong attosecond laser pulse with a general atom, i.e., beyond the models of quasi-one-electron or…

Atomic Physics · Physics 2016-11-17 X. Guan , O. Zatsarinny , K. Bartschat , B. I. Schneider , J. Feist , C. J. Noble

The present work explores quantitative limits to the Single-Active Electron (SAE) approximation, often used to deal with strong-field ionization and subsequent attosecond dynamics. Using a time-dependent multi\-configuration approach,…

Atomic Physics · Physics 2025-11-04 Jean-Nicolas Vigneau , Tung Nguyen-Dang , Eric Charron , Osman Atabek

We propose and computationally study a method for simultaneously orienting the angular momentum of asymmetric top molecules along: 1) a laboratory-fixed direction; 2) the molecular intermediate moment of inertia axis; 3) the laser field…

Quantum Physics · Physics 2022-11-21 Emil J. Zak
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