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We present a novel theory and implementation for computing coupled electronic and quantal nuclear subsystems on a single potential energy surface, moving beyond the standard Born-Oppenheimer (BO) separation of nuclei and electrons. We…

Chemical Physics · Physics 2021-11-15 Ziyong Chen , Jun Yang

We report a computational first-principles study of positron trapping at vacancy defects in metals and semiconductors. The main emphasis is on the energetics of the trapping process including the interplay between the positron state and the…

Materials Science · Physics 2007-08-19 I. Makkonen , M. J. Puska

The usefulness of the Relativistic Schr\"odinger Theory (RST) is studied in the field of atomic physics. As a concrete demonstration, the positronium groundstate is considered in great detail; especially the groundstate energy $E_0$ is…

High Energy Physics - Theory · Physics 2007-05-23 T. Beck , M. Mattes , M. Sorg

We have investigated the threshold of photodetachment of Li^- leading to the formation of the residual Li atom in the $2p ^2P$ state. The excited residual atom was selectively photoionized via an intermediate Rydberg state and the resulting…

We present first-principles calculations of the rate of energy exchanges between electrons and ions in nonequilibrium warm dense plasmas, liquid metals and hot solids, a fundamental property for which various models offer diverging…

Plasma Physics · Physics 2019-05-29 Jacopo Simoni , Jérôme Daligault

Large-scale relativistic configuration-interaction calculation of energy levels of core-excited states of lithium-like ions is presented. Quantum electrodynamic, nuclear recoil, and frequency-dependent Breit corrections are included in the…

Atomic Physics · Physics 2015-06-11 V. A. Yerokhin , A. Surzhykov

The multiconfiguration Dirac-Hartree-Fock method is applied to study the electron affinities of At and its homologous elements Cl, Br, and I. Our method of calculation is validated through the comparison with the available experimental…

Atomic Physics · Physics 2019-06-04 R. Si , C. Froese Fischer

We substantiate the need for account of the proper electromagnetic field of the electron in the canonical problem of hydrogen in relativistic quantum mechanics. From mathematical viewpoint, the goal is equivalent to determination of the…

Quantum Physics · Physics 2021-01-12 Leon V. Biguaa , Vladimir V. Kassandrov

We report the first measurements of the transverse ($P_{x}$ and $P_{y}$) and longitudinal ($P_{z}$) components of the polarization transfer to a bound proton in the deuteron via the $^{2}\mathrm{H}(\vec{e},e'\vec{p})$ reaction, over a wide…

Orientation effects on the resistivity of copper grain boundaries are studied systematically with two different atomistic tight binding methods. A methodology is developed to model the resistivity of grain boundaries using the Embedded Atom…

A low-energy storage ring with an ultracold electron cooler has been coupled with a heavy-ion accelerator facilitating high-resolution electron-ion collision spectroscopy of the heaviest few-electron ions. In the present work resonant…

New constraints for the nuclear equation of state at suprasaturation densities have been obtained by measuring collective particle flows in heavy-ion reactions at relativistic energies. Ratios and differences of neutron and hydrogen flows…

Nuclear Experiment · Physics 2018-02-13 W. Trautmann , H. H. Wolter

Energies of (3s2 3p6 3d9 4l4l'), (3s2 3p5 3d10 4l4l'), and (3s 3p6 3d10 4l4l') states for Cu-like ions with Z = 30 -100 are evaluated to second order in relativistic many-body perturbation theory (RMBPT) starting from a Ni-like Dirac-Fock…

Atomic Physics · Physics 2009-11-10 U. I. Safronova , W. R. Johnson , A. Shlyaptseva , S. Hamasha

We propose the cyclotron state retrieval of an electron trapped in a Penning trap by using different measurement schemes based on suitable modifications of the applied electromagnetic fields and exploiting the axial degree of freedom as a…

Quantum Physics · Physics 2009-10-30 Stefano Mancini , Paolo Tombesi

This article presents an overview of current understanding of the interaction of low-energy positrons with molecules with emphasis on resonances, positron attachment and annihilation. Annihilation rates measured as a function of positron…

Atomic Physics · Physics 2010-09-22 G. F. Gribakin , J. A. Young , C. M. Surko

The osmotic coefficient of solutions of rod-like polyelectrolytes is considered by comparing current theoretical treatments and simulations to recent experimental data. The discussion is restricted to the case of monovalent counterions and…

Soft Condensed Matter · Physics 2009-11-07 M. Deserno , C. Holm , J. Blaul , M. Ballauff , M. Rehahn

We report results of the calculation of the low-lying levels of neutral Si using a combination of the configuration interaction and many-body perturbation theory (CI+MBPT method). We treat Si I as an atom with four valence electrons and use…

Atomic Physics · Physics 2017-08-02 R. T. Imanbaeva , M. G. Kozlov , E. A. Konovalova

A survey of atomic binding energies used by general purpose Monte Carlo systems is reported. Various compilations of these parameters have been evaluated; their accuracy is estimated with respect to experimental data. Their effects on…

Computational Physics · Physics 2011-09-29 Maria Grazia Pia , Hee Seo , Matej Batic , Marcia Begalli , Chan Hyeong Kim , Lina Quintieri , Paolo Saracco

We compute corrections to the gyromagnetic factor of an electron bound in a hydrogen-like ion at order alpha^2(Z alpha)^5. This result removes a major uncertainty in predictions for silicon and carbon ions, used to determine the atomic mass…

Atomic Physics · Physics 2018-01-31 Andrzej Czarnecki , Matthew Dowling , Jan Piclum , Robert Szafron

We demonstrate that energy levels of excited states in a hydrogenic system consisting of an arbitrary nucleus and an antiproton can be calculated within the framework of nonrelativistic quantum electrodynamics, even for a large nuclear…

Atomic Physics · Physics 2025-09-10 V. Patkóš , K. Pachucki