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Positron binding to silver and gold atoms was studied using a fully {\it ab initio} relativistic method, which combines the configuration interaction method with many-body perturbation theory. It was found that the silver atom forms a bound…

Atomic Physics · Physics 2009-11-06 V. A. Dzuba , V. V. Flambaum , C. Harabati

A model-potential approach to calculating positron-molecule binding energies and annihilation rates is developed. Unlike existing ab initio calculations, which have mostly been applied to strongly polar molecules, the present methodology…

Atomic Physics · Physics 2018-12-31 A. R. Swann , G. F. Gribakin

Positron binding in parabenzoquinone is studied using \textit{ab initio} many-body theory. The effects of electron-positron correlations including polarization, virtual positronium formation and positron-hole repulsion, as well as those of…

Chemical Physics · Physics 2025-02-17 S. K. Gregg , J. Hofierka , B. Cunningham , D. G. Green

Calculations of the positron binding energies to all atoms in the periodic table are presented and atoms where the positron-atom binding actually exists are identified. The results of these calculations and accurate calculations of other…

Atomic Physics · Physics 2015-06-16 C. Harabati , V. A. Dzuba , V. V. Flambaum

We present relativistic many-body calculations of total electron binding energy of neutral atoms up to element $Z=120$. Binding energy for ions may be found by subtracting known ionization potentials. Accuracy of the results for $17<Z…

Atomic Physics · Physics 2025-03-25 V. A. Dzuba , V. V. Flambaum , A. V. Afanasjev

A model-potential approach has been developed to study positron interactions with molecules. Binding energies and annihilation rates are calculated for positron bound states with a range of alkane molecules, including rings and isomers. The…

Atomic Physics · Physics 2019-09-17 A. R. Swann , G. F. Gribakin

A many-body theory approach developed by the authors [Phys. Rev. A 70, 032720 (2004)] is applied to positron bound states and annihilation rates in atomic systems. Within the formalism, full account of virtual positronium (Ps) formation is…

Atomic Physics · Physics 2014-11-20 J. A. Ludlow , G. F. Gribakin

Relativistic coupled-cluster single-double approximation is used to calculate positron-atom bound states. The method is tested on closed-shell atoms such as Be, Mg, Ca, Zn, Cd, and Hg where a number of accurate calculations is available. It…

Atomic Physics · Physics 2015-06-04 V. A. Dzuba , V. V. Flambaum , G. F. Gribakin , C. Harabati

Predicted twenty years ago, positron binding to neutral atoms has not yet been observed experimentally. A new scheme is proposed to detect positron-atom bound states by colliding Rydberg positronium (Ps) with neutral atoms. Estimates of the…

Atomic Physics · Physics 2016-05-23 A. R. Swann , D. B. Cassidy , A. Deller , G. F. Gribakin

A method is proposed for detecting positron-atom bound states by observing enhanced positron annihilation due to electronic Feshbach resonances at electron-volt energies. The method is applicable to a range of open-shell transition metal…

Atomic Physics · Physics 2010-12-10 V. A. Dzuba , V. V. Flambaum , G. F. Gribakin

Positron binding energies in the negative ions H$^-$, F$^-$, Cl$^-$ and Br$^-$, and the closed-shell atoms Be, Mg, Zn and Ca, are calculated via a many-body theory approach developed by the authors [J.~Hofierka \emph{et al.} Nature~{\bf…

Atomic Physics · Physics 2023-11-23 J. Hofierka , B. Cunningham , C. M. Rawlins , C. H. Patterson , D. G. Green

Positrons bind to molecules leading to vibrational excitation and spectacularly enhanced annihilation. Whilst positron binding energies have been measured via resonant annihilation spectra for $\sim$90 molecules in the past two decades, an…

Atomic Physics · Physics 2023-03-23 J. Hofierka , B. Cunningham , C. M. Rawlins , C. H. Patterson , D. G. Green

Core-polarization interactions are investigated in low-energy electron elastic scattering from the atoms In,Sn,Eu,Au and At through the calculation of their electron affinities. The complex angular momentum method wherein is embedded the…

Atomic Physics · Physics 2015-10-07 Z. Felfli , A. Z. Msezane

The binding energies of the excited states of positronium are calculated using the two body Dirac equations of constraint formalism. The results from nonperturbative evaluation are compared to those from perturbative evaluation. The…

High Energy Physics - Phenomenology · Physics 2026-04-14 Robert W. Johnson

The model-potential approach previously developed by the authors to study positron interactions with molecules is used to calculate the positron binding energy for $n$-alkanes (C$_n$H$_{2n+2}$) and the corresponding cycloalkanes…

Atomic Physics · Physics 2020-11-13 A. R. Swann , G. F. Gribakin

We determine the binding energy of the negative positronium ion in the limits of one spatial dimension and of infinitely many dimensions. The numerical result for the one-dimensional ground state energy seems to be a rational number,…

High Energy Physics - Phenomenology · Physics 2012-01-30 Nikita Blinov , Andrzej Czarnecki

A many-body theory approach is developed for the problem of positron-atom scattering and annihilation. Strong electron-positron correlations are included non-perturbatively through the calculation of the electron-positron vertex function.…

Atomic Physics · Physics 2007-05-23 G. F. Gribakin , J. Ludlow

We develop a theoretical method within the framework of relativistic many-body theory to accurately treat correlation corrections in atoms with few valence electrons. This method combines the all-order approach currently used in precision…

Atomic Physics · Physics 2009-09-01 M. S. Safronova , M. G. Kozlov , W. R. Johnson , Dansha Jiang

Thermal corrections, including relativistic effects, for the positronium atom are discussed. The theoretical description of thermal corrections is carried out within the framework of relativistic quantum electrodynamics. As a result,…

Atomic Physics · Physics 2022-03-14 D. Solovyev , T. Zalialiutdinov , A. Anikin

We present the positron coupled cluster singles and doubles (POS-CCSD) method to calculate positron binding energies in molecules. This framework treats electrons and positrons on an equal footing and includes up to simultaneous…

Chemical Physics · Physics 2026-03-23 Rosario R. Riso , Jan Haakon M. Trabski , Federico Rossi , Dermot Green , Henrik Koch
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